Manipulation of Charge Dynamics for Efficient and Bright Blue Perovskite Light-Emitting Diodes with Chiral Ligands

© 2023 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 35(2023), 38 vom: 27. Sept., Seite e2302059
1. Verfasser: Zhang, Lingjiao (VerfasserIn)
Weitere Verfasser: Hu, Sujuan, Guo, Min, Ren, Yunfei, Wei, Linfeng, Li, Wenxuan, Lin, Faxu, Yang, Zhiyong, Yang, Zhenyu, Liu, Chuan, Liu, Baiquan
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article blue emission displays high efficiency light-emitting diodes perovskites
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520 |a Perovskite light-emitting diodes (PeLEDs) emerge as a promising class of optoelectronic devices for next-generation displays and lighting technology. However, the performance of blue PeLEDs lags far behind that of their green and red counterparts, including the unachieved trade-off between high efficiency and high luminance, severe efficiency roll-off, and unsatisfactory power efficiency. Here, a multi-functional chiral ligand of L-phenylalanine methyl ester hydrochloride is strategically introduced into quasi-2D perovskites, which can effectively passivate defects, modulate the phase distribution, improve photoluminescence quantum yield, guarantee high-quality film morphology, and enhance charge transport. Furthermore, ladder-like hole transport layers are established, boosting charge injection and balance. The resultant sky-blue PeLEDs (the photoluminescence peak is 493 nm and the electroluminescence peak is 497 nm) exhibit an external quantum efficiency of 12.43% at 1000 cd m-2 and a record power efficiency of 18.42 lm W-1 , rendering that the performance is among the best blue PeLEDs 
650 4 |a Journal Article 
650 4 |a blue emission 
650 4 |a displays 
650 4 |a high efficiency 
650 4 |a light-emitting diodes 
650 4 |a perovskites 
700 1 |a Hu, Sujuan  |e verfasserin  |4 aut 
700 1 |a Guo, Min  |e verfasserin  |4 aut 
700 1 |a Ren, Yunfei  |e verfasserin  |4 aut 
700 1 |a Wei, Linfeng  |e verfasserin  |4 aut 
700 1 |a Li, Wenxuan  |e verfasserin  |4 aut 
700 1 |a Lin, Faxu  |e verfasserin  |4 aut 
700 1 |a Yang, Zhiyong  |e verfasserin  |4 aut 
700 1 |a Yang, Zhenyu  |e verfasserin  |4 aut 
700 1 |a Liu, Chuan  |e verfasserin  |4 aut 
700 1 |a Liu, Baiquan  |e verfasserin  |4 aut 
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773 1 8 |g volume:35  |g year:2023  |g number:38  |g day:27  |g month:09  |g pages:e2302059 
856 4 0 |u http://dx.doi.org/10.1002/adma.202302059  |3 Volltext 
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