Controllable Synthesis of 2H-1T' Mox Re(1- x ) S2 Lateral Heterostructures and Their Tunable Optoelectronic Properties

© 2023 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 35(2023), 38 vom: 06. Sept., Seite e2304171
1. Verfasser: Sun, Xiaona (VerfasserIn)
Weitere Verfasser: Liu, Yang, Shi, Jianwei, Si, Chen, Du, Jiantao, Liu, Xinfeng, Jiang, Chengbao, Yang, Shengxue
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article MoxRe(1-x)S2 alloys chemical vapor deposition heterostructures photodetectors
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520 |a Constructing heterostructures and doping are valid ways to improve the optoelectronic properties of transition metal dichalcogenides (TMDs) and optimize the performance of TMDs-based photodetectors. Compared with transfer techniques, chemical vapor deposition (CVD) has higher efficiency in preparing heterostructures. As for the one-step CVD growth of heterostructures, cross-contamination between the two materials may occur during the growth process, which may provide the possibility of one-step simultaneous realization of controllable doping and formation of alloy-based heterostructures by finely tuning the growth dynamics. Here, 2H-1T' Mox Re(1- x ) S2 alloy-to-alloy lateral heterostructures are synthesized through this one-step CVD growth method, utilizing the cross-contamination and different growth temperatures of the two alloys. Due to the doping of a small amount of Re atoms in 2H MoS2 , 2H Mox Re(1- x ) S2 has a high response rejection ratio in the solar-blind ultraviolet (SBUV) region and exhibits a positive photoconductive (PPC) effect. While the 1T' Mox Re(1- x ) S2 formed by heavily doping Mo atoms into 1T' ReS2 will produce a negative photoconductivity (NPC) effect under UV laser irradiation. The optoelectronic property of 2H-1T' Mox Re(1- x ) S2 -based heterostructures can be modulated by gate voltage. These findings are expected to expand the functionality of traditional optoelectronic devices and have potential applications in optoelectronic logic devices 
650 4 |a Journal Article 
650 4 |a MoxRe(1-x)S2 alloys 
650 4 |a chemical vapor deposition 
650 4 |a heterostructures 
650 4 |a photodetectors 
700 1 |a Liu, Yang  |e verfasserin  |4 aut 
700 1 |a Shi, Jianwei  |e verfasserin  |4 aut 
700 1 |a Si, Chen  |e verfasserin  |4 aut 
700 1 |a Du, Jiantao  |e verfasserin  |4 aut 
700 1 |a Liu, Xinfeng  |e verfasserin  |4 aut 
700 1 |a Jiang, Chengbao  |e verfasserin  |4 aut 
700 1 |a Yang, Shengxue  |e verfasserin  |4 aut 
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773 1 8 |g volume:35  |g year:2023  |g number:38  |g day:06  |g month:09  |g pages:e2304171 
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