|
|
|
|
| LEADER |
01000caa a22002652c 4500 |
| 001 |
NLM357712781 |
| 003 |
DE-627 |
| 005 |
20250304205212.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
231226s2023 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.202303523
|2 doi
|
| 028 |
5 |
2 |
|a pubmed25n1192.xml
|
| 035 |
|
|
|a (DE-627)NLM357712781
|
| 035 |
|
|
|a (NLM)37269248
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Xia, Yi
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Enhanced Free-Radical Generation on MoS2 /Pt by Light and Water Vapor Co-Activation for Selective CO Detection with High Sensitivity
|
| 264 |
|
1 |
|c 2023
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Revised 27.07.2023
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2023 Wiley-VCH GmbH.
|
| 520 |
|
|
|a Semiconductor-based gas sensors hold great promise for effective carbon monoxide (CO) detection. However, boosting sensor response and selectivity remains a key priority in moist conditions. In this study, a composite material, Pt quantum dots decorated MoS2 nanosheets (MoS2 /Pt), is developed as a highly sensitive material for CO detection when facilitated with visible light. The MoS2 /Pt sensor shows a significantly improved response (87.4%) with impressive response/recovery kinetics (20 s/17 s), long-term stability (60 days), and good selectivity to CO at high humidity (≈60%). It is confirmed both experimentally and theoretically that the MoS2 /Pt surface lowers the activation energy to convert CO to CO2 via the free radicals induced by the synergy of photochemical effects and water vapor. As a result, the MoS2 /Pt surface promotes both CO response and selectivity, providing fundamental clues to improve room-temperature semiconductor-based sensors for gas detection under extreme conditions
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a MoS2/Pt
|
| 650 |
|
4 |
|a free radicals
|
| 650 |
|
4 |
|a light
|
| 650 |
|
4 |
|a selective CO sensing
|
| 650 |
|
4 |
|a water vapor
|
| 700 |
1 |
|
|a Guo, Shenghui
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Yang, Li
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a He, Sufang
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zhou, Liexing
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Wang, Mingjun
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Gao, Jiyun
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Hou, Ming
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Wang, Jing
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Komarneni, Sridhar
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 30 vom: 03. Juli, Seite e2303523
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnas
|
| 773 |
1 |
8 |
|g volume:35
|g year:2023
|g number:30
|g day:03
|g month:07
|g pages:e2303523
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.202303523
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 35
|j 2023
|e 30
|b 03
|c 07
|h e2303523
|