Strong Tough Thermogalvanic Hydrogel Thermocell With Extraordinarily High Thermoelectric Performance

© 2023 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 35(2023), 32 vom: 04. Aug., Seite e2300696
1. Verfasser: Liu, Lili (VerfasserIn)
Weitere Verfasser: Zhang, Ding, Bai, Peijia, Mao, Yin, Li, Qi, Guo, Jiaqi, Fang, Yanjie, Ma, Rujun
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article strength stretchable thermogalvanic thermocells stretching-induced crystallization thermal energy harvesting toughness wearable devices
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520 |a Thermocells can continuously convert heat into electricity, and they are widely used to power wearable electronic devices. However, they have a risk of leakage and poor mechanical properties. Although quasi-solid ionic thermocells can overcome the issue of electrolyte leakage, the trade-off between their excellent mechanical properties and high thermopower remains a major challenge. In this study, stretching-induced crystallization and the thermoelectric effect are combined to propose a high-strength quasi-solid stretchable polyvinyl alcohol thermogalvanic thermocell (SPTC) with a large tensile strength of 19 MPa and high thermopower of 6.5 mV K-1 . The SPTC exhibits a high stretchability of 1300%, ultrahigh toughness of 163.4 MJ m-3 , and high specific output power density of 1969 µW m-2  K-2 . These comprehensive properties are superior to those of previously reported quasi-solid stretchable thermogalvanic thermocells. The use of SPTC-based systems in wearable devices for energy-autonomous strain sensors and health monitoring is demonstrated. This can facilitate the rapid implementation of sustainable wearable electronics in the Internet of Things era 
650 4 |a Journal Article 
650 4 |a strength 
650 4 |a stretchable thermogalvanic thermocells 
650 4 |a stretching-induced crystallization 
650 4 |a thermal energy harvesting 
650 4 |a toughness 
650 4 |a wearable devices 
700 1 |a Zhang, Ding  |e verfasserin  |4 aut 
700 1 |a Bai, Peijia  |e verfasserin  |4 aut 
700 1 |a Mao, Yin  |e verfasserin  |4 aut 
700 1 |a Li, Qi  |e verfasserin  |4 aut 
700 1 |a Guo, Jiaqi  |e verfasserin  |4 aut 
700 1 |a Fang, Yanjie  |e verfasserin  |4 aut 
700 1 |a Ma, Rujun  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Advanced materials (Deerfield Beach, Fla.)  |d 1998  |g 35(2023), 32 vom: 04. Aug., Seite e2300696  |w (DE-627)NLM098206397  |x 1521-4095  |7 nnns 
773 1 8 |g volume:35  |g year:2023  |g number:32  |g day:04  |g month:08  |g pages:e2300696 
856 4 0 |u http://dx.doi.org/10.1002/adma.202300696  |3 Volltext 
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