Ce/Pumice and Ni/Pumice as heterogeneous catalysts for syngas production from biomass gasification

Copyright © 2023 The Author(s). Published by Elsevier Ltd.. All rights reserved.

Bibliographische Detailangaben
Veröffentlicht in:Waste management (New York, N.Y.). - 1999. - 166(2023) vom: 01. Juli, Seite 270-279
1. Verfasser: Señorans, S (VerfasserIn)
Weitere Verfasser: R-Díaz, J, Escalante, D, González, L A, Díaz, L
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Waste management (New York, N.Y.)
Schlagworte:Journal Article Biomass Gasification Heterogeneous catalyst Pennisetum setaceum Pumice Syngas pumice NT5NN5KL16 Gases Silicates
LEADER 01000caa a22002652c 4500
001 NLM357101006
003 DE-627
005 20250304192522.0
007 cr uuu---uuuuu
008 231226s2023 xx |||||o 00| ||eng c
024 7 |a 10.1016/j.wasman.2023.05.017  |2 doi 
028 5 2 |a pubmed25n1190.xml 
035 |a (DE-627)NLM357101006 
035 |a (NLM)37207588 
035 |a (PII)S0956-053X(23)00358-6 
040 |a DE-627  |b ger  |c DE-627  |e rakwb 
041 |a eng 
100 1 |a Señorans, S  |e verfasserin  |4 aut 
245 1 0 |a Ce/Pumice and Ni/Pumice as heterogeneous catalysts for syngas production from biomass gasification 
264 1 |c 2023 
336 |a Text  |b txt  |2 rdacontent 
337 |a ƒaComputermedien  |b c  |2 rdamedia 
338 |a ƒa Online-Ressource  |b cr  |2 rdacarrier 
500 |a Date Completed 05.06.2023 
500 |a Date Revised 05.06.2023 
500 |a published: Print-Electronic 
500 |a Citation Status MEDLINE 
520 |a Copyright © 2023 The Author(s). Published by Elsevier Ltd.. All rights reserved. 
520 |a This work presents a study of synthesis and characterization of catalysts-based cerium and nickel supported on the pumice stone (Ce/Pumice and Ni/Pumice) to be used in the gasification process of an invasive species present in the Canary Islands, such as Pennisetum setaceum to obtain syngas. Specifically, the effect of the metal impregnated on the pumice, and the effect of catalyst on the gasification process was studied. For this purpose, the composition of the gas was determined and the results obtained were compared with those obtained in non-catalytic thermochemical processes. Gasification tests were performed using a simultaneous thermal analyzer coupled with a mass spectrometer, providing a detailed analysis of the gases released during the process. The results showed that during the catalytic gasification process of the Pennisetum setaceum, the gases produced appear at lower temperatures in the catalytic process that in the non-catalytic process. Specifically, H2 appears at 640.42 °C and 641.84 °C when Ce/pumice and Ni/pumice were used as catalyst, respectively, compared to 697.41 °C for the non-catalytic process. Moreover, the reactivity at 50 % of char conversion for the catalytic process (0.34 and 0.38 min-1 for Ce/pumice and Ni/pumice, respectively) was higher than for the non-catalytic process (0.28 min-1), indicating that the incorporation of Ce and Ni on the pumitic material increases the gasification rate of the char compared to the pumitic support. Catalytic biomass gasification is an innovative technology that can provide new opportunities for research and development of renewable energy technologies, as well as for the creation of green jobs 
650 4 |a Journal Article 
650 4 |a Biomass 
650 4 |a Gasification 
650 4 |a Heterogeneous catalyst 
650 4 |a Pennisetum setaceum 
650 4 |a Pumice 
650 4 |a Syngas 
650 7 |a pumice  |2 NLM 
650 7 |a NT5NN5KL16  |2 NLM 
650 7 |a Gases  |2 NLM 
650 7 |a Silicates  |2 NLM 
700 1 |a R-Díaz, J  |e verfasserin  |4 aut 
700 1 |a Escalante, D  |e verfasserin  |4 aut 
700 1 |a González, L A  |e verfasserin  |4 aut 
700 1 |a Díaz, L  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Waste management (New York, N.Y.)  |d 1999  |g 166(2023) vom: 01. Juli, Seite 270-279  |w (DE-627)NLM098197061  |x 1879-2456  |7 nnas 
773 1 8 |g volume:166  |g year:2023  |g day:01  |g month:07  |g pages:270-279 
856 4 0 |u http://dx.doi.org/10.1016/j.wasman.2023.05.017  |3 Volltext 
912 |a GBV_USEFLAG_A 
912 |a SYSFLAG_A 
912 |a GBV_NLM 
912 |a GBV_ILN_350 
951 |a AR 
952 |d 166  |j 2023  |b 01  |c 07  |h 270-279