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20231226071758.0 |
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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202302732
|2 doi
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|a pubmed24n1190.xml
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|a (NLM)37203431
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|a DE-627
|b ger
|c DE-627
|e rakwb
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| 041 |
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|a eng
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| 100 |
1 |
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|a Zhang, Yufeng
|e verfasserin
|4 aut
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| 245 |
1 |
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|a Sequential-Stimuli Induced Stepwise-Response of Pyridylpyrenes
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 11.08.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a Stimuli-responsive materials, especially multi-stimuli-responsive materials, can sense external stimuli such as light, heat, and force, have shown great potential in drug delivery, data storage, encryption, energy-harvesting, and artificial intelligence. Conventional multi-stimuli-responsive materials are sensitive to each independent stimulus, causing losses in the diversity and accuracy of the identification for practical application. Herein, a unique phenomenon of sequential-stimuli induced stepwise-response generated from elaborately designed single-component organic materials is reported, which shows large bathochromic shifts up to 5800 cm-1 under sequential stimuli of force and light. In contrast to multi-stimuli-responsive materials, the response of these materials strictly relies on the sequence of stimuli, allowing logicality, rigidity, and accuracy to be integrated into one single-component material. The molecular keypad lock is built based on these materials, pointing promising to a future for this logical response in significant practical applications. This breakthrough gives a new drive to classical stimuli-responsiveness and provides a fundamental design strategy for new generations of high-performance stimuli-responsive materials
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|a Journal Article
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|a UV light
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|a bathochromic shift
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| 650 |
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|a mechanical force
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|a molecular keypad lock
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4 |
|a sequential-stimuli induced stepwise-response
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| 700 |
1 |
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|a Zhang, Shuai
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Liang, Chen
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Shi, Junqing
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Ji, Lei
|e verfasserin
|4 aut
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| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 32 vom: 02. Aug., Seite e2302732
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:35
|g year:2023
|g number:32
|g day:02
|g month:08
|g pages:e2302732
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| 856 |
4 |
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|u http://dx.doi.org/10.1002/adma.202302732
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