Room-Temperature Synthesis of Carbon Dot/TiO2 Composites with High Photocatalytic Activity

Benefiting from the wide-range absorption and adjustable energy gap, carbon dots (C-dots) have attracted a great deal of attention and they have been used to sensitize semiconductor nanocomposites to boost the efficiency of energy conversion devices, while there is still a lack of fundamental unders...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1999. - 39(2023), 20 vom: 23. Mai, Seite 7184-7191
1. Verfasser: Zhou, Hao (VerfasserIn)
Weitere Verfasser: Zhang, Bin, Jiang, Zhan, Zhao, Haiguang, Zhang, Yuanming
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article
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520 |a Benefiting from the wide-range absorption and adjustable energy gap, carbon dots (C-dots) have attracted a great deal of attention and they have been used to sensitize semiconductor nanocomposites to boost the efficiency of energy conversion devices, while there is still a lack of fundamental understanding of the interaction between such materials and their influence on the catalytic activity on the reaction process. In this study, C-dots were used to modify TiO2 to form a direct Z-scheme (DZS) junction for enhancement of the photocatalytic activity. The C-dot/TiO2 composite was prepared by ultrasonication at room temperature through coupling between the Ti-O-C bond and electrostatic interaction. The C-dots can dramatically enhance the absorption of the composite by forming the DZS, and the composite is enabled to generate more free radicals, which facilitate ∼10 times higher photocatalytic activity compared to that of TiO2. As a proof of concept, the as-prepared C-dot/TiO2 was used for textile wastewater dye degradation. This study provides an efficient approach for room-temperature preparation of C-dot/TiO2 composites with high photocatalytic activity 
650 4 |a Journal Article 
700 1 |a Zhang, Bin  |e verfasserin  |4 aut 
700 1 |a Jiang, Zhan  |e verfasserin  |4 aut 
700 1 |a Zhao, Haiguang  |e verfasserin  |4 aut 
700 1 |a Zhang, Yuanming  |e verfasserin  |4 aut 
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