A novel strategy for efficient utilization of manganese tailings : High SO2 resistance SCR catalyst preparation and faujasite zeolite synthesis

Copyright © 2023 Elsevier Ltd. All rights reserved.

Bibliographische Detailangaben
Veröffentlicht in:Waste management (New York, N.Y.). - 1999. - 164(2023) vom: 01. Juni, Seite 66-73
1. Verfasser: Wu, Hongli (VerfasserIn)
Weitere Verfasser: Liu, Weizao, Zhang, Xiaogang, Liu, Qingcai
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Waste management (New York, N.Y.)
Schlagworte:Journal Article Core–shell structure Faujasite zeolite Manganese tailings NH(3)-SCR SO(2) resistance Manganese 42Z2K6ZL8P faujasite Zeolites mehr... 1318-02-1 Ammonia 7664-41-7
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520 |a Herein, a core-shell structure SiO2Mn catalyst was successfully synthesized from manganese tailings for NO removal through selective catalytic reduction with ammonia at low temperature. In the presence of 10 % H2O and 100 ppm SO2, the SiO2@Mn catalyst exhibited excellent catalytic activity of 85 % NO conversion at 225 °C. This special core-shell was constructed by inert nano-SiO2 particles, which grew and encapsulated on the surface of manganese oxide, inhibiting the reaction between SO2 with MnOx and thus improving the SO2 resistance. Furthermore, a filter residue was generated in the process of catalysts preparation. Under proper hydrothermal conditions, the residue comprising of Si, Al, and O was used to synthesize high-crystallinity X-type zeolite. This process fully utilized manganese tailings and inspired for Mn-based catalysts design and X-type zeolite preparation, realizing the dual benefits of atmosphere purification and solid waste disposal 
650 4 |a Journal Article 
650 4 |a Core–shell structure 
650 4 |a Faujasite zeolite 
650 4 |a Manganese tailings 
650 4 |a NH(3)-SCR 
650 4 |a SO(2) resistance 
650 7 |a Manganese  |2 NLM 
650 7 |a 42Z2K6ZL8P  |2 NLM 
650 7 |a faujasite  |2 NLM 
650 7 |a Zeolites  |2 NLM 
650 7 |a 1318-02-1  |2 NLM 
650 7 |a Ammonia  |2 NLM 
650 7 |a 7664-41-7  |2 NLM 
700 1 |a Liu, Weizao  |e verfasserin  |4 aut 
700 1 |a Zhang, Xiaogang  |e verfasserin  |4 aut 
700 1 |a Liu, Qingcai  |e verfasserin  |4 aut 
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856 4 0 |u http://dx.doi.org/10.1016/j.wasman.2023.03.038  |3 Volltext 
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