|
|
|
|
| LEADER |
01000naa a22002652 4500 |
| 001 |
NLM355270307 |
| 003 |
DE-627 |
| 005 |
20231226064009.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
231226s2023 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.202301406
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n1184.xml
|
| 035 |
|
|
|a (DE-627)NLM355270307
|
| 035 |
|
|
|a (NLM)37022336
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Wu, Haodi
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Mechanochemical Synthesis of High-Entropy Perovskite toward Highly Sensitive and Stable X-ray Flat-Panel Detectors
|
| 264 |
|
1 |
|c 2023
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Revised 20.07.2023
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2023 Wiley-VCH GmbH.
|
| 520 |
|
|
|a Perovskites are attracting attention for optoelectronic devices. Despite their promise, the large-scale synthesis of perovskite materials with exact stoichiometry, especially high-entropy perovskites, has been a major challenge. Moreover, the difficulty in stoichiometry control also hinders the development of perovskite X-ray flat-panel detectors. Previous reports all employed simple MAPbI3 as the active layer, while the performance still falls short of optimized single-crystal-based single-pixel detectors. Herein, a scalable and universal strategy of a mechanochemical method is adopted to synthesize stoichiometric high-entropy perovskite powders with high quality and high quantity (>1 kg per batch). By utilizing these stoichiometric perovskites, the first FA0.9 MA0.05 Cs0.05 Pb(I0.9 Br0.1 )3 -based X-ray flat-panel detector with low trap density and large mobility-lifetime product (7.5 × 10-3 cm2 V-1 ) is reported. The assembled panel detector exhibits close-to-single-crystal performance (high sensitivity of 2.1 × 104 µC Gyair -1 cm-2 and ultralow detection limit of 1.25 nGyair s-1 ), high spatial resolution of 0.46 lp/pixel, as well as excellent thermal robustness under industrial standards. The high performance in the high-entropy perovskite-based X-ray FPDs has the potential to facilitate the development of new-generation X-ray-detection systems
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a X-ray flat-panel detectors
|
| 650 |
|
4 |
|a high-entropy perovskites
|
| 650 |
|
4 |
|a mechanochemistry
|
| 700 |
1 |
|
|a Chen, Xu
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Song, Zihao
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zhang, Ao
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Du, Xinyuan
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a He, Xin
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Wang, Hanqi
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Xu, Ling
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zheng, Zhiping
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Niu, Guangda
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Tang, Jiang
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 29 vom: 18. Juli, Seite e2301406
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:35
|g year:2023
|g number:29
|g day:18
|g month:07
|g pages:e2301406
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.202301406
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 35
|j 2023
|e 29
|b 18
|c 07
|h e2301406
|