Polymeric Memristor Based Artificial Synapses with Ultra-Wide Operating Temperature

© 2023 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 35(2023), 23 vom: 01. Juni, Seite e2209728
1. Verfasser: Li, Jiayu (VerfasserIn)
Weitere Verfasser: Qian, Yangzhou, Li, Wen, Yu, Songcheng, Ke, Yunxin, Qian, Haowen, Lin, Yen-Hung, Hou, Cheng-Hung, Shyue, Jing-Jong, Zhou, Jia, Chen, Ye, Xu, Jiangping, Zhu, Jintao, Yi, Mingdong, Huang, Wei
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article memristors neuromorphic computing operational stability organic semiconductors solution process
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520 |a Neuromorphic electronics, being inspired by how the brain works, hold great promise to the successful implementation of smart artificial systems. Among several neuromorphic hardware issues, a robust device functionality under extreme temperature is of particular importance for practical applications. Given that the organic memristors for artificial synapse applications are demonstrated under room temperature, achieving a robust device performance at extremely low or high temperature is still utterly challenging. In this work, the temperature issue is addressed by tuning the functionality of the solution-based organic polymeric memristor. The optimized memristor demonstrates a reliable performance under both the cryogenic and high-temperature environments. The unencapsulated organic polymeric memristor shows a robust memristive response under test temperature ranging from 77 to 573 K. Utilizing X-ray photoelectron spectroscopy (XPS) and time-of-flight secondary-ion mass spectrometry (ToF-SIMS) depth profiling, the device working mechanism is unveiled by comparing the compositional profiles of the fresh and written organic polymeric memristors. A reversible ion migration induced by an applied voltage contributes to the characteristic switching behavior of the memristor. Herein, both the robust memristive response achieved at extreme temperatures and the verified device working mechanism will remarkably accelerate the development of memristors in neuromorphic systems 
650 4 |a Journal Article 
650 4 |a memristors 
650 4 |a neuromorphic computing 
650 4 |a operational stability 
650 4 |a organic semiconductors 
650 4 |a solution process 
700 1 |a Qian, Yangzhou  |e verfasserin  |4 aut 
700 1 |a Li, Wen  |e verfasserin  |4 aut 
700 1 |a Yu, Songcheng  |e verfasserin  |4 aut 
700 1 |a Ke, Yunxin  |e verfasserin  |4 aut 
700 1 |a Qian, Haowen  |e verfasserin  |4 aut 
700 1 |a Lin, Yen-Hung  |e verfasserin  |4 aut 
700 1 |a Hou, Cheng-Hung  |e verfasserin  |4 aut 
700 1 |a Shyue, Jing-Jong  |e verfasserin  |4 aut 
700 1 |a Zhou, Jia  |e verfasserin  |4 aut 
700 1 |a Chen, Ye  |e verfasserin  |4 aut 
700 1 |a Xu, Jiangping  |e verfasserin  |4 aut 
700 1 |a Zhu, Jintao  |e verfasserin  |4 aut 
700 1 |a Yi, Mingdong  |e verfasserin  |4 aut 
700 1 |a Huang, Wei  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Advanced materials (Deerfield Beach, Fla.)  |d 1998  |g 35(2023), 23 vom: 01. Juni, Seite e2209728  |w (DE-627)NLM098206397  |x 1521-4095  |7 nnns 
773 1 8 |g volume:35  |g year:2023  |g number:23  |g day:01  |g month:06  |g pages:e2209728 
856 4 0 |u http://dx.doi.org/10.1002/adma.202209728  |3 Volltext 
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