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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202301218
|2 doi
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|a pubmed24n1181.xml
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|a (DE-627)NLM354456067
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|a (NLM)36940232
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Ma, Hongyun
|e verfasserin
|4 aut
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|a A Biocompatible Supercapacitor Diode with Enhanced Rectification Capability toward Ion/Electron-Coupling Logic Operations
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 22.06.2023
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|a Date Revised 22.06.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a The main challenge faced by the forthcoming human-computer interaction is that biological systems and electronic devices adopt two different information carriers, i.e., ions and electrons, respectively. To bridge the gap between these two systems, developing ion/electron-coupling devices for logic operation is a feasible and effective approach. Accordingly, herein a supercapacitor-based ionic diode (CAPode) that takes electrochemically amorphized molybdenum oxide as the working electrode is developed. Benefiting from its unique size and charge dual ion-sieving effects, the molybdenum oxide electrode exhibits a record-high rectification ratio of 136, which is over 10 times higher than those of reported systems. It also delivers an ultrahigh specific capacitance of 448 F g⁻1 and an excellent cycling stability of up to 20 000 cycles, greatly outperforming those of previous works. These excellent rectification capability and electrochemical performances allow the as-built CAPode to work well in AND and OR logic gates, validating great potential in ion/electron-coupling logic operations. More attractively, the superior biocompatibilities of molybdenum oxide and relevant constituent materials enable the constructed CAPode to be applied as bioelectronics without regard to biosafety, paving a new way toward forthcoming human-computer interaction
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|a Journal Article
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|a human-computer interaction
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|a ion-sieving effect
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|a logic operation
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|a molybdenum oxide
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|a supercapacitor diodes
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|a Liang, Jie
|e verfasserin
|4 aut
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|a Qiu, Jian
|e verfasserin
|4 aut
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|a Jiang, Li
|e verfasserin
|4 aut
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|a Ma, Lingxiao
|e verfasserin
|4 aut
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|a Sheng, Hongwei
|e verfasserin
|4 aut
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|a Shao, Mingjiao
|e verfasserin
|4 aut
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|a Wang, Qi
|e verfasserin
|4 aut
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|a Li, Fengfeng
|e verfasserin
|4 aut
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|a Fu, Yujun
|e verfasserin
|4 aut
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|a Wang, Jing
|e verfasserin
|4 aut
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|a Xie, Erqing
|e verfasserin
|4 aut
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|a Chai, Yang
|e verfasserin
|4 aut
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|a Lan, Wei
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 25 vom: 15. Juni, Seite e2301218
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:35
|g year:2023
|g number:25
|g day:15
|g month:06
|g pages:e2301218
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|u http://dx.doi.org/10.1002/adma.202301218
|3 Volltext
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|d 35
|j 2023
|e 25
|b 15
|c 06
|h e2301218
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