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|a 10.1002/adma.202208947
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|a pubmed24n1181.xml
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|a (DE-627)NLM354382942
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|a (NLM)36932897
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|a DE-627
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|c DE-627
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|a eng
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|a Wu, Xiaojun
|e verfasserin
|4 aut
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|a Generation of 13.9-mJ Terahertz Radiation from Lithium Niobate Materials
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 08.06.2023
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|a Date Revised 08.06.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a Extremely strong-field terahertz (THz) radiation in free space has compelling applications in nonequilibrium condensed matter state regulation, all-optical THz electron acceleration and manipulation, THz biological effects, etc. However, these practical applications are constrained by the absence of high-intensity, high-efficiency, high-beam-quality, and stable solid-state THz light sources. Here, the generation of single-cycle 13.9-mJ extreme THz pulses from cryogenically cooled lithium niobate crystals and a 1.2% energy conversion efficiency from 800 nm to THz are demonstrated experimentally using the tilted pulse-front technique driven by a home-built 30-fs, 1.2-Joule Ti:sapphire laser amplifier. The focused peak electric field strength is estimated to be 7.5 MV cm-1 . A record of 1.1-mJ THz single-pulse energy at a 450 mJ pump at room temperature is produced and observed that the self-phase modulation of the optical pump can induce THz saturation behavior from the crystals in the substantially nonlinear pump regime. This study lays the foundation for the generation of sub-Joule THz radiation from lithium niobate crystals and will inspire more innovations in extreme THz science and applications
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|a Journal Article
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|a nonlinear optics
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|a terahertz generation
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|a tilted pulse-front technique
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|a ultrafast phenomena
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|a Kong, Deyin
|e verfasserin
|4 aut
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|a Hao, Sibo
|e verfasserin
|4 aut
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|a Zeng, Yushan
|e verfasserin
|4 aut
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|a Yu, Xieqiu
|e verfasserin
|4 aut
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|a Zhang, Baolong
|e verfasserin
|4 aut
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|a Dai, Mingcong
|e verfasserin
|4 aut
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|a Liu, Shaojie
|e verfasserin
|4 aut
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|a Wang, Jiaqi
|e verfasserin
|4 aut
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|a Ren, Zejun
|e verfasserin
|4 aut
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|a Chen, Sai
|e verfasserin
|4 aut
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|a Sang, Jianhua
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|4 aut
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|a Wang, Kang
|e verfasserin
|4 aut
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|a Zhang, Dongdong
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|4 aut
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|a Liu, Zhongkai
|e verfasserin
|4 aut
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|a Gui, Jiayan
|e verfasserin
|4 aut
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|a Yang, Xiaojun
|e verfasserin
|4 aut
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|a Xu, Yi
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|4 aut
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|a Leng, Yuxin
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|4 aut
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|a Li, Yutong
|e verfasserin
|4 aut
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|a Song, Liwei
|e verfasserin
|4 aut
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|a Tian, Ye
|e verfasserin
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|a Li, Ruxin
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 23 vom: 14. Juni, Seite e2208947
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:35
|g year:2023
|g number:23
|g day:14
|g month:06
|g pages:e2208947
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|u http://dx.doi.org/10.1002/adma.202208947
|3 Volltext
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