Generation of 13.9-mJ Terahertz Radiation from Lithium Niobate Materials

© 2023 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 35(2023), 23 vom: 14. Juni, Seite e2208947
1. Verfasser: Wu, Xiaojun (VerfasserIn)
Weitere Verfasser: Kong, Deyin, Hao, Sibo, Zeng, Yushan, Yu, Xieqiu, Zhang, Baolong, Dai, Mingcong, Liu, Shaojie, Wang, Jiaqi, Ren, Zejun, Chen, Sai, Sang, Jianhua, Wang, Kang, Zhang, Dongdong, Liu, Zhongkai, Gui, Jiayan, Yang, Xiaojun, Xu, Yi, Leng, Yuxin, Li, Yutong, Song, Liwei, Tian, Ye, Li, Ruxin
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article nonlinear optics terahertz generation tilted pulse-front technique ultrafast phenomena
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520 |a Extremely strong-field terahertz (THz) radiation in free space has compelling applications in nonequilibrium condensed matter state regulation, all-optical THz electron acceleration and manipulation, THz biological effects, etc. However, these practical applications are constrained by the absence of high-intensity, high-efficiency, high-beam-quality, and stable solid-state THz light sources. Here, the generation of single-cycle 13.9-mJ extreme THz pulses from cryogenically cooled lithium niobate crystals and a 1.2% energy conversion efficiency from 800 nm to THz are demonstrated experimentally using the tilted pulse-front technique driven by a home-built 30-fs, 1.2-Joule Ti:sapphire laser amplifier. The focused peak electric field strength is estimated to be 7.5 MV cm-1 . A record of 1.1-mJ THz single-pulse energy at a 450 mJ pump at room temperature is produced and observed that the self-phase modulation of the optical pump can induce THz saturation behavior from the crystals in the substantially nonlinear pump regime. This study lays the foundation for the generation of sub-Joule THz radiation from lithium niobate crystals and will inspire more innovations in extreme THz science and applications 
650 4 |a Journal Article 
650 4 |a nonlinear optics 
650 4 |a terahertz generation 
650 4 |a tilted pulse-front technique 
650 4 |a ultrafast phenomena 
700 1 |a Kong, Deyin  |e verfasserin  |4 aut 
700 1 |a Hao, Sibo  |e verfasserin  |4 aut 
700 1 |a Zeng, Yushan  |e verfasserin  |4 aut 
700 1 |a Yu, Xieqiu  |e verfasserin  |4 aut 
700 1 |a Zhang, Baolong  |e verfasserin  |4 aut 
700 1 |a Dai, Mingcong  |e verfasserin  |4 aut 
700 1 |a Liu, Shaojie  |e verfasserin  |4 aut 
700 1 |a Wang, Jiaqi  |e verfasserin  |4 aut 
700 1 |a Ren, Zejun  |e verfasserin  |4 aut 
700 1 |a Chen, Sai  |e verfasserin  |4 aut 
700 1 |a Sang, Jianhua  |e verfasserin  |4 aut 
700 1 |a Wang, Kang  |e verfasserin  |4 aut 
700 1 |a Zhang, Dongdong  |e verfasserin  |4 aut 
700 1 |a Liu, Zhongkai  |e verfasserin  |4 aut 
700 1 |a Gui, Jiayan  |e verfasserin  |4 aut 
700 1 |a Yang, Xiaojun  |e verfasserin  |4 aut 
700 1 |a Xu, Yi  |e verfasserin  |4 aut 
700 1 |a Leng, Yuxin  |e verfasserin  |4 aut 
700 1 |a Li, Yutong  |e verfasserin  |4 aut 
700 1 |a Song, Liwei  |e verfasserin  |4 aut 
700 1 |a Tian, Ye  |e verfasserin  |4 aut 
700 1 |a Li, Ruxin  |e verfasserin  |4 aut 
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773 1 8 |g volume:35  |g year:2023  |g number:23  |g day:14  |g month:06  |g pages:e2208947 
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