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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202212258
|2 doi
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|a pubmed24n1178.xml
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|a (DE-627)NLM353470511
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|a (NLM)36840924
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Niu, Benfang
|e verfasserin
|4 aut
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|a Multifunctional Hybrid Interfacial Layers for High-Performance Inverted Perovskite Solar Cells
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Completed 25.05.2023
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|a Date Revised 25.05.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a Challenges remain hindering the performance and stability of inverted perovskite solar cells (PSCs), particularly for the nonstable interface between lead halide perovskite and charge extraction metal oxide layer. Herein, a simple yet scalable interfacial strategy to facilitate the assemble of high-performance inverted PSCs and scale-up modules is reported. The hybrid interfacial layer containing self-assembly triphenylamine and conjugated poly(arylamine) simultaneously improves the chemical stability, charge extraction, and energy level alignment of hole-selective interface, meanwhile promoting perovskite crystallization. Consequently, the correspondent inverted PSCs and modules achieve remarkable power conversion efficiencies (PCEs) of 24.5% and 20.7% (aperture area of 19.4 cm2 ), respectively. The PSCs maintain over 80% of its initial efficiency under one-sun equivalent illumination of 1200 h. This strategy is also effective to perovskite with various bandgaps, demonstrating the highest PCE of 19.6% for the 1.76-eV bandgap PSCs. Overall, this work provides a simple yet scalable interfacial strategy for obtaining state-of-the-art inverted PSCs and modules
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|a Journal Article
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|a interface
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|a metal oxide
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|a passivation
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|a perovskite solar cells
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|a self-assembled molecule
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|a Liu, Haoran
|e verfasserin
|4 aut
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|a Huang, Yanchun
|e verfasserin
|4 aut
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|a Gu, Emely
|e verfasserin
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|a Yan, Minxing
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|a Shen, Ziqiu
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|a Yan, Kangrong
|e verfasserin
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|a Yan, Buyi
|e verfasserin
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|a Yao, Jizhong
|e verfasserin
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|a Fang, Yanjun
|e verfasserin
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|a Chen, Hongzheng
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|a Li, Chang-Zhi
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 21 vom: 19. Mai, Seite e2212258
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:35
|g year:2023
|g number:21
|g day:19
|g month:05
|g pages:e2212258
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|u http://dx.doi.org/10.1002/adma.202212258
|3 Volltext
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