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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202211523
|2 doi
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|a pubmed25n1176.xml
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|a (DE-627)NLM353137898
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|a (NLM)36807415
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|a DE-627
|b ger
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|e rakwb
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|a eng
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|a Zhou, Huijie
|e verfasserin
|4 aut
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|a Ethanol-Induced Ni2+ -Intercalated Cobalt Organic Frameworks on Vanadium Pentoxide for Synergistically Enhancing the Performance of 3D-Printed Micro-Supercapacitors
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 11.05.2023
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|a Date Revised 11.05.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a The synthesis of metal-organic framework (MOF) nanocomposites with high energy density and excellent mechanical strength is limited by the degree of lattice matching and crystal surface structure. In this study, dodecahedral ZIF-67 is synthesized uniformly on vanadium pentoxide nanowires. The influence of the coordination mode on the surface of ZIF-67 in ethanol is also investigated. Benefitting from the different coordination abilities of Ni2+ , Co2+ , and N atoms, spatially separated surface-active sites are created through metal-ion exchange. Furthermore, the incompatibility between the d8 electronic configuration of Ni2+ and the three-dimensional (3D) structure of ZIF-67 afforded the synthesis of hollow structures by controlling the amount of Ni doping. The formation of NiCo-MOFCoOOH@V2 O5 nanocomposites is confirmed using X-ray absorption fine structure analysis. The high performance of the obtained composite is illustrated by fabricating a 3D-printed micro-supercapacitor, exhibiting a high area specific capacitance of 585 mF cm-2 and energy density of 159.23 µWh cm-2 (at power density = 0.34 mW cm-2 ). The solvent/coordination tuning strategy demonstrated in this study provides a new direction for the synthesis of high-performance nanomaterials for electrochemical energy storage applications
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|a Journal Article
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|a 3D printing
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|a ethanol-induced
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|a metal-organic framework
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|a micro-supercapacitor
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|a nanocomposite
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|a Zhu, Guoyin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Dong, Shengyang
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Liu, Pin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Lu, Yiyao
|e verfasserin
|4 aut
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| 700 |
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|a Zhou, Zhen
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Cao, Shuai
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhang, Yizhou
|e verfasserin
|4 aut
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| 700 |
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|a Pang, Huan
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 19 vom: 21. Mai, Seite e2211523
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnas
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| 773 |
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|g volume:35
|g year:2023
|g number:19
|g day:21
|g month:05
|g pages:e2211523
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|u http://dx.doi.org/10.1002/adma.202211523
|3 Volltext
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