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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202207883
|2 doi
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|a pubmed25n1170.xml
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|a (DE-627)NLM351102485
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|a (NLM)36599055
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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| 100 |
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|a Luo, Xin
|e verfasserin
|4 aut
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|a Efficient Perovskite/Silicon Tandem Solar Cells on Industrially Compatible Textured Silicon
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Completed 02.03.2023
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|a Date Revised 02.03.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a Monolithic perovskite/silicon tandem solar cells promise power-conversion efficiencies (PCEs) exceeding the Shockley-Queisser limit of single-junction solar cells. The conformal deposition of perovskites on industrially feasible textured silicon solar cells allows for both lowered manufacturing costs and a higher matched photocurrent density, compared to state-of-the-art tandems using front-side flat or mildly textured silicon. However, the inferior crystal quality of perovskite films grown on fully-textured silicon compromises the photovoltaic performance. Here, an anion-engineered additive strategy is developed to control the crystallization process of wide-bandgap perovskite films, which enables improved film crystallinity, reduced trap density, and conformal deposition on industrially textured silicon. This strategy allows the fabrication of 28.6%-efficient perovskite/silicon heterojunction tandem solar cells (certified 27.9%, 1 cm2 ). This approach is compatible with the scalable fabrication of tandems on industrially textured silicon, demonstrating an efficiency of 25.1% for an aperture area of 16 cm2 . The anion-engineered additive significantly improves the operating stability of wide-bandgap perovskite solar cells, and the encapsulated tandem solar cells retain over 80% of their initial performance following 2000 h of operation under full 1-sun illumination in ambient conditions
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|a Journal Article
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|a anion-engineered additive strategy
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|a hybrid two-step perovskite deposition
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|a industrially feasible textured silicon
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|a perovskite/silicon tandem solar cells
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1 |
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|a Luo, Haowen
|e verfasserin
|4 aut
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1 |
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|a Li, Hongjiang
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Xia, Rui
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zheng, Xuntian
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Huang, Zilong
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Liu, Zhou
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Gao, Han
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhang, Xueling
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Li, Songlin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Feng, Zhiqiang
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Chen, Yifeng
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Tan, Hairen
|e verfasserin
|4 aut
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| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 9 vom: 18. März, Seite e2207883
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnas
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| 773 |
1 |
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|g volume:35
|g year:2023
|g number:9
|g day:18
|g month:03
|g pages:e2207883
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| 856 |
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|u http://dx.doi.org/10.1002/adma.202207883
|3 Volltext
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