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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202209475
|2 doi
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|a pubmed24n1169.xml
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|a DE-627
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|e rakwb
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|a eng
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|a López-Magano, Alberto
|e verfasserin
|4 aut
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|a Recent Advances in the Use of Covalent Organic Frameworks as Heterogenous Photocatalysts in Organic Synthesis
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|c 2023
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|a Text
|b txt
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|a ƒaComputermedien
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|a ƒa Online-Ressource
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|a Date Completed 15.06.2023
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|a Date Revised 15.06.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 The Authors. Advanced Materials published by Wiley-VCH GmbH.
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|a Organic photochemistry is intensely developed in the 1980s, in which the nature of excited electronic states and the energy and electron transfer processes are thoroughly studied and finally well-understood. This knowledge from molecular organic photochemistry can be transferred to the design of covalent organic frameworks (COFs) as active visible-light photocatalysts. COFs constitute a new class of crystalline porous materials with substantial application potentials. Featured with outstanding structural tunability, large porosity, high surface area, excellent stability, and unique photoelectronic properties, COFs are studied as potential candidates in various research areas (e.g., photocatalysis). This review aims to provide the state-of-the-art insights into the design of COF photocatalysts (pristine, functionalized, and hybrid COFs) for organic transformations. The catalytic reaction mechanism of COF-based photocatalysts and the influence of dimensionality and crystallinity on heterogenous photocatalysis performance are also discussed, followed by perspectives and prospects on the main challenges and opportunities in future research of COFs and COF-based photocatalysts
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|a Journal Article
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|a Review
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|a covalent organic frameworks
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|a photocatalysis
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|a porous organic polymers
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|a reaction mechanism
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|a selective organic reactions
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|a Daliran, Saba
|e verfasserin
|4 aut
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|a Oveisi, Ali Reza
|e verfasserin
|4 aut
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|a Mas-Ballesté, Rubén
|e verfasserin
|4 aut
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|a Dhakshinamoorthy, Amarajothi
|e verfasserin
|4 aut
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|a Alemán, José
|e verfasserin
|4 aut
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|a Garcia, Hermenegildo
|e verfasserin
|4 aut
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| 700 |
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|a Luque, Rafael
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 24 vom: 22. Juni, Seite e2209475
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|x 1521-4095
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|g volume:35
|g year:2023
|g number:24
|g day:22
|g month:06
|g pages:e2209475
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|u http://dx.doi.org/10.1002/adma.202209475
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