|
|
|
|
| LEADER |
01000naa a22002652 4500 |
| 001 |
NLM348675275 |
| 003 |
DE-627 |
| 005 |
20231226040825.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
231226s2023 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.202207617
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n1162.xml
|
| 035 |
|
|
|a (DE-627)NLM348675275
|
| 035 |
|
|
|a (NLM)36353914
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Liang, Fang-Cheng
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Synergistic Effect of Cation Composition Engineering of Hybrid Cs1-x FAx PbBr3 Nanocrystals for Self-Healing Electronics Application
|
| 264 |
|
1 |
|c 2023
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Completed 02.03.2023
|
| 500 |
|
|
|a Date Revised 02.03.2023
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2023 Wiley-VCH GmbH.
|
| 520 |
|
|
|a Mixed-cation hybrid perovskite nanocrystal (HPNC) with high crystallinity, color purity, and tunable optical bandgap offers a practical pathway toward next-generation displays. Herein, a two-step modified hot-injection combined with cation compositional engineering and surface treatment to synthesize high-purity cesium/formamidinium lead bromide HPNCs(Cs1-x FAx PbBr3 ) is presented. The optimized Cs0.5 FA0.5 PbBr3 light-emitting devices (LEDs) exhibit uniform luminescence of 3500 cd m-2 and a prominent current efficiency of 21.5 cd A-1 . As a proof of concept, a self-healing polymer (SHP) integrated with white LED backlight and laser prototypes exhibited 4 h autonomous self-healing through the synergistic effect of weak reversible imine bonds and stronger H-bonds. First, the SHP-HPNCs-initial and SHP-HPNCs-cut possess high long-term stability and dramatically suppressed lead leakage as low as 0.6 ppm along with a low leakage rate of 1.11 × 10-5 cm2 and 3.36 × 10-5 cm2 even over 6 months in water. Second, the Cs0.5 FA0.5 PbBr3 HPNCs and SHP-induced shattered-repaired perovskite glass substrate show the lowest lasing threshold values of 1.24 and 8.58 µJ cm-2 , respectively. This work provides an integrative and in-depth approach to exploiting SHP with intrinsic and entropic self-healing capabilities combined with HPNCs to develop robust and reliable soft-electronic backlight and laser applications
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a A-site cations
|
| 650 |
|
4 |
|a laser
|
| 650 |
|
4 |
|a light-emitting diodes
|
| 650 |
|
4 |
|a nanocrystals
|
| 650 |
|
4 |
|a self-healing
|
| 650 |
|
4 |
|a soft-electronic backlight
|
| 700 |
1 |
|
|a Jhuang, Fu-Cheng
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Fang, Yu-Han
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Benas, Jean-Sebastien
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Chen, Wei-Cheng
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Yan, Zhen-Li
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Lin, Wei-Chun
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Su, Chun-Jen
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Sato, Yuki
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Chiba, Takayuki
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Kido, Junji
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Kuo, Chi-Ching
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 9 vom: 10. März, Seite e2207617
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:35
|g year:2023
|g number:9
|g day:10
|g month:03
|g pages:e2207617
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.202207617
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 35
|j 2023
|e 9
|b 10
|c 03
|h e2207617
|