Emergent Magnetic States and Tunable Exchange Bias at 3d Nitride Heterointerfaces

Bibliographische Detailangaben
Veröffentlicht in:	Advanced materials (Deerfield Beach, Fla.). - 1998. - 35(2023), 2 vom: 23. Jan., Seite e2208221
1. Verfasser:	Jin, Qiao (VerfasserIn)
Weitere Verfasser:	Zhang, Qinghua, Bai, He, Huon, Amanda, Charlton, Timothy, Chen, Shengru, Lin, Shan, Hong, Haitao, Cui, Ting, Wang, Can, Guo, Haizhong, Gu, Lin, Zhu, Tao, Fitzsimmons, Michael R, Jin, Kui-Juan, Wang, Shanmin, Guo, Er-Jia
Format:	Online-Aufsatz
Sprache:	English
Veröffentlicht:	2023
Zugriff auf das übergeordnete Werk:	Advanced materials (Deerfield Beach, Fla.)
Schlagworte:	Journal Article Fe3N cylinder diameter engineering exchange bias magnetic anisotropy

Beschreibung
Zusammenfassung:	© 2022 Wiley-VCH GmbH. Interfacial magnetism stimulates the discovery of giant magnetoresistance (MR) and spin-orbital coupling across the heterointerfaces, facilitating the intimate correlation between spin transport and complex magnetic structures. Over decades, functional heterointerfaces composed of nitrides have seldom been explored due to the difficulty in synthesizing high-quality nitride films with correct compositions. Here, the fabrication of single-crystalline ferromagnetic Fe3 N thin films with precisely controlled thicknesses is reported. As film thickness decreases, the magnetization dramatically deteriorates, and the electronic state changes from metallic to insulating. Strikingly, the high-temperature ferromagnetism is maintained in a Fe3 N layer with a thickness down to 2 u.c. (≈8 Å). The MR exhibits a strong in-plane anisotropy; meanwhile, the anomalous Hall resistivity reverses its sign when the Fe3 N layer thickness exceeds 5 u.c. Furthermore, a sizable exchange bias is observed at the interfaces between a ferromagnetic Fe3 N and an antiferromagnetic CrN. The exchange bias field and saturation moment strongly depend on the controllable bending curvature using the cylinder diameter engineering technique, implying the tunable magnetic states under lattice deformation. This work provides a guideline for exploring functional nitride films and applying their interfacial phenomena for innovative perspectives toward practical applications
Beschreibung:	Date Completed 13.01.2023 Date Revised 13.01.2023 published: Print-Electronic Citation Status PubMed-not-MEDLINE
ISSN:	1521-4095
DOI:	10.1002/adma.202208221