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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202207908
|2 doi
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|a pubmed24n1158.xml
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|a (NLM)36245304
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|a DE-627
|b ger
|c DE-627
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|a eng
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|a Wang, Dongdong
|e verfasserin
|4 aut
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|a Rational Screening of Artificial Solid Electrolyte Interphases on Zn for Ultrahigh-Rate and Long-Life Aqueous Batteries
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 13.01.2023
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|a Date Revised 13.01.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2022 Wiley-VCH GmbH.
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|a Solid electrolyte interphase (SEI) on Zn anodes plays a pivotal role for high-rate and long-life aqueous batteries, because it effectively inhibits side reactions and dendritic growth. Many materials are explored as SEIs by a trial-and-error approach. Herein, an exercisable way is proposed to screen the potential SEIs on Zn anodes in view of dendrite-suppressing ability and charge-transfer property theoretically. As an output of this screening, Zn3 (BO3 )2 (ZBO) is checked experimentally. In symmetrical cells, ZnZBO runs over 250 h at an ultrahigh current density of 50 mA cm-2 for a large areal capacity 10 mAh cm-2 . In full cells, Zn@ZBO||MnO2 shows an impressive cumulative capacity (≈406 mAh cm-2 ) under harsh conditions, i.e., a lean electrolyte condition (10 µL mAh-1 ), limited Zn supply (negative/positive electrode capacity ratio, N/P ratio = 2.3), and high areal capacity (5.0 mAh cm-2 ). The significance of this work lies in not only the first report of ZBO on Zn showing excellent electrochemical performance, but also a feasible way to screen the promising SEI materials for other metal anodes
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|a Journal Article
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|a Zn metal
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|a borates
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|a electrochemical performance
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|a solid electrolyte interphase
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|a Liu, Hongxia
|e verfasserin
|4 aut
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1 |
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|a Lv, Dan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wang, Cheng
|e verfasserin
|4 aut
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|a Yang, Jian
|e verfasserin
|4 aut
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|a Qian, Yitai
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 2 vom: 15. Jan., Seite e2207908
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:35
|g year:2023
|g number:2
|g day:15
|g month:01
|g pages:e2207908
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|u http://dx.doi.org/10.1002/adma.202207908
|3 Volltext
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