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231226s2022 xx |||||o 00| ||eng c |
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|a 10.1021/acs.langmuir.2c02011
|2 doi
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|a pubmed24n1156.xml
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|a (NLM)36191260
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|e rakwb
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|a eng
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| 100 |
1 |
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|a Wang, Shuai
|e verfasserin
|4 aut
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|a Rational Design of a Low-Dimensional and Metal-free Heterostructure for Efficient Water Oxidation
|b DFT and Experimental Studies
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|c 2022
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 18.10.2022
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a A nitrogen-doped fullerene dimer is synthesized and compounded with multi-walled carbon nanotubes (MWCNTs) to construct a low-dimensional and metal-free 0D-1D heterostructure for electrocatalytic water oxidation. The (C59N)2/MWCNTs heterostructure exhibits a highly efficient performance, as verified by both first-principles density functional theory and experimental studies. The *O → *OOH process is confirmed as the rate-determining step of water oxidation. The negatively charged N-doping leads to electronic redistribution and intermolecular charge transfer and thus reduces the uphill free energies of intermediates on the (C59N)2/MWCNTs interface. Therefore, the (C59N)2/MWCNTs heterostructure has great potential to emit light and heat in metal-free-based electrocatalytic water oxidation
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|a Journal Article
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|a Zhao, Rui
|e verfasserin
|4 aut
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|a Zheng, Tian
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Lu, Zheng
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Fang, Yuan
|e verfasserin
|4 aut
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| 700 |
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|a Xie, Haijiao
|e verfasserin
|4 aut
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| 700 |
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|a Wang, Wenjian
|e verfasserin
|4 aut
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| 700 |
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|a Xue, Weidong
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1999
|g 38(2022), 41 vom: 18. Okt., Seite 12562-12569
|w (DE-627)NLM098181009
|x 1520-5827
|7 nnns
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| 773 |
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|g volume:38
|g year:2022
|g number:41
|g day:18
|g month:10
|g pages:12562-12569
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|u http://dx.doi.org/10.1021/acs.langmuir.2c02011
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