Spontaneous Charging of Drops on Lubricant-Infused Surfaces
When a drop of a polar liquid slides over a hydrophobic surface, it acquires a charge. As a result, the surface charges oppositely. For applications such as the generation of electric energy, lubricant-infused surfaces (LIS) may be important because they show a low friction for drops. However, slide...
| Veröffentlicht in: | Langmuir : the ACS journal of surfaces and colloids. - 1992. - 38(2022), 41 vom: 18. Okt., Seite 12610-12616 |
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| 1. Verfasser: | |
| Weitere Verfasser: | , , , |
| Format: | Online-Aufsatz |
| Sprache: | English |
| Veröffentlicht: |
2022
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| Zugriff auf das übergeordnete Werk: | Langmuir : the ACS journal of surfaces and colloids |
| Schlagworte: | Journal Article |
| Zusammenfassung: | When a drop of a polar liquid slides over a hydrophobic surface, it acquires a charge. As a result, the surface charges oppositely. For applications such as the generation of electric energy, lubricant-infused surfaces (LIS) may be important because they show a low friction for drops. However, slide electrification on LIS has not been studied yet. Here, slide electrification on lubricant-infused surfaces was studied by measuring the charge generated by series of water drops sliding down inclined surfaces. As LIS, we used PDMS-coated glass with micrometer-thick silicone oil films on top. For PDMS-coated glass without lubricant, the charge for the first drop is highest. Then it decreases and saturates at a steady state charge per drop. With lubricant, the drop charge starts from 0, then it increases and reaches a maximum charge per drop. Afterward, it decreases again before reaching its steady-state value. This dependency is not a unique phenomenon for lubricant-infused PDMS; it also occurs on lubricant-infused micropillar surfaces. We attribute this dependency of charge on drop numbers to a change in surface conductivity and depletion of lubricant. These findings are helpful for understanding the charge process and optimizing solid-liquid nanogenerator devices in applications |
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| Beschreibung: | Date Revised 22.10.2022 published: Print-Electronic Citation Status PubMed-not-MEDLINE |
| ISSN: | 1520-5827 |
| DOI: | 10.1021/acs.langmuir.2c02085 |