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231226s2022 xx |||||o 00| ||eng c |
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|a 10.1021/acs.langmuir.2c01885
|2 doi
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|a eng
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|a Xiong, Jingjing
|e verfasserin
|4 aut
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|a Regulating Surface Wettability and Charge Density of Porous Carbon Particles by In Situ Growth of Polyaniline for Constructing an Efficient Electrical Percolation Network in Flow-Electrode Capacitive Deionization
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|c 2022
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|a Text
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|a ƒaComputermedien
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|a ƒa Online-Ressource
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|a Date Revised 11.10.2022
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a Both electrical conductivity and surface wettability are required for the selection of active carbon materials in flow-electrode capacitive deionization, while a trade-off exists between these two properties. In this work, a hybrid material with a thin layer of polyaniline (PANI) coating on activated carbon (AC/PANI) was successfully developed to retain excellent electrical conductivity and acquire good surface wettability. By adjusting the dosage of initiator, AC/PANI composites with different loading fractions of PANI were obtained. The electrochemical testing demonstrated that the AC/PANI composites have higher specific capacitance and lower ion diffusion resistance compared to pure AC, resulting in better desalinization performance. Specifically, with a feed concentration of 1600 mg/L, excellent adsorption capacity and high charge efficiency can be simultaneously achieved at 13.51 mg/g and 92.21%, respectively. Benefiting from the formation of a continuous electrical percolation network and reduced solid/liquid interfacial transport resistance, a 39% enhancement of average salt adsorption rate (from 0.54 to 0.75 μmol/min/cm2) was obtained
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|a Journal Article
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|a Zhu, Zetao
|e verfasserin
|4 aut
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|a Ye, Wenkai
|e verfasserin
|4 aut
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|a Mu, Liwen
|e verfasserin
|4 aut
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|a Lu, Xiaohua
|e verfasserin
|4 aut
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|a Zhu, Jiahua
|e verfasserin
|4 aut
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1985
|g 38(2022), 40 vom: 11. Okt., Seite 12263-12272
|w (DE-627)NLM098181009
|x 1520-5827
|7 nnas
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|g volume:38
|g year:2022
|g number:40
|g day:11
|g month:10
|g pages:12263-12272
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|u http://dx.doi.org/10.1021/acs.langmuir.2c01885
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