|
|
|
|
| LEADER |
01000naa a22002652 4500 |
| 001 |
NLM345189639 |
| 003 |
DE-627 |
| 005 |
20231226024512.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
231226s2022 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.202205261
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n1150.xml
|
| 035 |
|
|
|a (DE-627)NLM345189639
|
| 035 |
|
|
|a (NLM)36000490
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Ollearo, Riccardo
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Multidimensional Perovskites for High Detectivity Photodiodes
|
| 264 |
|
1 |
|c 2022
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Revised 06.10.2022
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2022 The Authors. Advanced Materials published by Wiley-VCH GmbH.
|
| 520 |
|
|
|a Low-dimensional perovskites attract increasing interest due to tunable optoelectronic properties and high stability. Here, it is shown that perovskite thin films with a vertical gradient in dimensionality result in graded electronic bandgap structures that are ideal for photodiode applications. Positioning low-dimensional, vertically-oriented perovskite phases at the interface with the electron blocking layer increases the activation energy for thermal charge generation and thereby effectively lowers the dark current density to a record-low value of 5 × 10-9 mA cm-2 without compromising responsivity, resulting in a noise-current-based specific detectivity exceeding 7 × 1012 Jones at 600 nm. These multidimensional perovskite photodiodes show promising air stability and a dynamic range over ten orders of magnitude, and thus represent a new generation of high-performance low-cost photodiodes
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a 2D perovskites
|
| 650 |
|
4 |
|a dark current
|
| 650 |
|
4 |
|a perovskites
|
| 650 |
|
4 |
|a photodiodes
|
| 700 |
1 |
|
|a Caiazzo, Alessandro
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Li, Junyu
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Fattori, Marco
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a van Breemen, Albert J J M
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Wienk, Martijn M
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Gelinck, Gerwin H
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Janssen, René A J
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 34(2022), 40 vom: 24. Okt., Seite e2205261
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:34
|g year:2022
|g number:40
|g day:24
|g month:10
|g pages:e2205261
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.202205261
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 34
|j 2022
|e 40
|b 24
|c 10
|h e2205261
|