Red Perovskite Light-Emitting Diodes with Efficiency Exceeding 25% Realized by Co-Spacer Cations

© 2022 Wiley-VCH GmbH.

Détails bibliographiques
Publié dans:Advanced materials (Deerfield Beach, Fla.). - 1998. - 34(2022), 36 vom: 27. Sept., Seite e2204460
Auteur principal: Jiang, Ji (Auteur)
Autres auteurs: Chu, Zema, Yin, Zhigang, Li, Jingzhen, Yang, Yingguo, Chen, Jingren, Wu, Jinliang, You, Jingbi, Zhang, Xingwang
Format: Article en ligne
Langue:English
Publié: 2022
Accès à la collection:Advanced materials (Deerfield Beach, Fla.)
Sujets:Journal Article co-spacer cations electroluminescence light-emitting diodes quasi-2D perovskites
Description
Résumé:© 2022 Wiley-VCH GmbH.
Perovskite light-emitting diodes (PeLEDs) have received great attention in recent years due to their narrow emission bandwidth and tunable emission spectrum. Efficient red emission is one of most important parts for lighting and displays. Quasi-2D perovskites can deliver high emission efficiency due to the strong carrier confinement, while the external quantum efficiencies (EQE) of red quasi-2D PeLEDs are inefficient at present, which is due to the complex distribution of different n-value phases in quasi-2D perovskite films. In this work, the phase distribution of the quasi-2D perovskite is finely controlled by mixing two different large organic cations, which effectively reduces the amount of smaller n-index phases, meanwhile the passivation of lead and halide defects in perovskite films is realized. Accordingly, the PeLEDs show 25.8% EQE and 1300 cd m-2 maximum brightness at 680 nm, which exhibits the highest performance for red PeLEDs up to now
Description:Date Revised 08.09.2022
published: Print-Electronic
Citation Status PubMed-not-MEDLINE
ISSN:1521-4095
DOI:10.1002/adma.202204460