High-throughput nuclear resonance time domain interferometry using annular slits

open access.

Bibliographische Detailangaben
Veröffentlicht in:Journal of synchrotron radiation. - 1994. - 29(2022), Pt 3 vom: 01. Mai, Seite 677-686
1. Verfasser: Pavlik, Marc (VerfasserIn)
Weitere Verfasser: Brown, Dennis E, Hu, Michael Y, Zhao, Jiyong, Lurio, Laurence, Alp, E Ercan
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2022
Zugriff auf das übergeordnete Werk:Journal of synchrotron radiation
Schlagworte:Journal Article Kohlrausch–Williams–Watts model annular slits momentum transfers nuclear resonance time domain interferometry relaxation times
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520 |a Nuclear resonance time domain interferometry (NR-TDI) is used to study the slow dynamics of liquids (that do not require Mössbauer isotopes) at atomic and molecular length scales. Here the TDI method of using a stationary two-line magnetized 57Fe foil as a source and a stationary single-line stainless steel foil analyzer is employed. The new technique of adding an annular slit in front of a single silicon avalanche photodiode detector enables a wide range of momentum transfers (1 to 100 nm-1 by varying the distance between the annular slits and sample) with a high count rate of up to 160 Hz with a Δq resolution of ±1.7 nm-1 at q = 14 nm-1. The sensitivity of this method in determining relaxation times is quantified and discussed. The Kohlrausch-Williams-Watts (KWW) model was used to extract relaxation times for glycerol. These relaxation times give insight into the dynamics of the electron density fluctuations of glycerol as a function of temperature and momentum transfers 
650 4 |a Journal Article 
650 4 |a Kohlrausch–Williams–Watts model 
650 4 |a annular slits 
650 4 |a momentum transfers 
650 4 |a nuclear resonance time domain interferometry 
650 4 |a relaxation times 
700 1 |a Brown, Dennis E  |e verfasserin  |4 aut 
700 1 |a Hu, Michael Y  |e verfasserin  |4 aut 
700 1 |a Zhao, Jiyong  |e verfasserin  |4 aut 
700 1 |a Lurio, Laurence  |e verfasserin  |4 aut 
700 1 |a Alp, E Ercan  |e verfasserin  |4 aut 
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773 1 8 |g volume:29  |g year:2022  |g number:Pt 3  |g day:01  |g month:05  |g pages:677-686 
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