A Self-Assembled 3D Penetrating Nanonetwork for High-Performance Intrinsically Stretchable Polymer Light-Emitting Diodes
© 2022 Wiley-VCH GmbH.
| Veröffentlicht in: | Advanced materials (Deerfield Beach, Fla.). - 1998. - 34(2022), 27 vom: 18. Juli, Seite e2201844 |
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| Weitere Verfasser: | , , , , , , , |
| Format: | Online-Aufsatz |
| Sprache: | English |
| Veröffentlicht: |
2022
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| Zugriff auf das übergeordnete Werk: | Advanced materials (Deerfield Beach, Fla.) |
| Schlagworte: | Journal Article 3D penetrating nanonetworks intrinsically stretchable materials polymer light-emitting diodes self-assembly |
| Zusammenfassung: | © 2022 Wiley-VCH GmbH. The emergence of wearable technology can significantly benefit from electronic displays fabricated using intrinsically stretchable (is-) materials. Typically, an improvement in the stretchability of conventional light-emitting polymers is accompanied by a decrease in charge transportability, thus resulting in a significant decrease in device efficiency. In this study, a self-assembled 3D penetrating nanonetwork is developed to achieve increased stretchability and mobility simultaneously, based on high-molecular-weight phenylenevinylene (L-SY-PPV) and polyacrylonitrile (PAN). The mobility of L-SY-PPV/PAN increases by 5-6 times and the stretchability increases from 20% (pristine L-SY-PPV film) to 100%. A high current efficiency (CE) of 8.13 cd A-1 is observed in polymer light-emitting diodes (PLEDs) fabricated using 40% stretched L-SY-PPV/PAN. Furthermore, using a polyethyleneimine ethoxylated (PEIE), an 1,10-phenanthroline monohydrate (pBphen), and a reduced Triton X-100 (TR) chelated Zn-based is- electron-injection layer of Zn-PEIE-pBphen-TR, an is-PLED is realized with a turn-on voltage of 6.5 V and a high CE of 2.35 cd A-1 . These results demonstrate the effectiveness of using the self-assembled 3D penetrating nanonetwork for the fabrication of is-PLEDs |
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| Beschreibung: | Date Revised 07.07.2022 published: Print-Electronic Citation Status PubMed-not-MEDLINE |
| ISSN: | 1521-4095 |
| DOI: | 10.1002/adma.202201844 |