Adaptive Self-Organization of Nanomaterials Enables Strain-Insensitive Resistance of Stretchable Metallic Nanocomposites

© 2022 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 34(2022), 23 vom: 16. Juni, Seite e2200980
1. Verfasser: Jung, Dongjun (VerfasserIn)
Weitere Verfasser: Lim, Chaehong, Park, Chansul, Kim, Yeongjun, Kim, Minseong, Lee, Seunghwan, Lee, Hyunjin, Kim, Jeong Hyun, Hyeon, Taeghwan, Kim, Dae-Hyeong
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2022
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article metallic nanocomposites self-organization of nanomaterials skin electronics strain-insensitive resistance stretchable conductors
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520 |a Highly conductive and stretchable nanocomposites are promising material candidates for skin electronics. However, the resistance of stretchable metallic nanocomposites highly depends on external strains, often deteriorating the performance of fabricated electronic devices. Here, a material strategy for the highly conductive and stretchable nanocomposites comprising metal nanomaterials of various dimensions and a viscoelastic block-copolymer matrix is presented. The resistance of the nanocomposites can be well retained under skin deformations (<50% strain). It is demonstrated that silver nanomaterials can self-organize inside the viscoelastic media in response to external strain when their surface is conjugated with 1-decanethiol. Distinct self-organization behaviors associated with nanomaterial dimensions and strain conditions are found. Adopting the optimum composition of 0D/1D/2D silver nanomaterials can render the resistance of the nanocomposites insensitive to uniaxial or biaxial strains. As a result, the resistance can be maintained with a variance of < 1% during 1000 stretching cycles under uniaxial and biaxial strains of <50% while a high conductivity of ≈31 000 S cm-1 is achieved 
650 4 |a Journal Article 
650 4 |a metallic nanocomposites 
650 4 |a self-organization of nanomaterials 
650 4 |a skin electronics 
650 4 |a strain-insensitive resistance 
650 4 |a stretchable conductors 
700 1 |a Lim, Chaehong  |e verfasserin  |4 aut 
700 1 |a Park, Chansul  |e verfasserin  |4 aut 
700 1 |a Kim, Yeongjun  |e verfasserin  |4 aut 
700 1 |a Kim, Minseong  |e verfasserin  |4 aut 
700 1 |a Lee, Seunghwan  |e verfasserin  |4 aut 
700 1 |a Lee, Hyunjin  |e verfasserin  |4 aut 
700 1 |a Kim, Jeong Hyun  |e verfasserin  |4 aut 
700 1 |a Hyeon, Taeghwan  |e verfasserin  |4 aut 
700 1 |a Kim, Dae-Hyeong  |e verfasserin  |4 aut 
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773 1 8 |g volume:34  |g year:2022  |g number:23  |g day:16  |g month:06  |g pages:e2200980 
856 4 0 |u http://dx.doi.org/10.1002/adma.202200980  |3 Volltext 
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