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231226s2022 xx |||||o 00| ||eng c |
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|a 10.1021/acs.langmuir.1c03428
|2 doi
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|a pubmed24n1127.xml
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|a (NLM)35289631
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|e rakwb
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|a eng
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| 100 |
1 |
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|a Lv, Lingling
|e verfasserin
|4 aut
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| 245 |
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|a Priority Occupation of C-Sites by N-Confining P-Implantation in Pyrrodic N-Sites in NCNTP,N-Mo2C for Highly Efficient Electrocatalytic Hydrogen Evolution
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|c 2022
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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| 338 |
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Revised 29.03.2022
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a Optimizing the electronic configuration of Mo2C by activating heteroatom(s)-neighboring carbon atoms to enhance the activity of hydrogen evolution reaction (HER) has been demonstrated. However, the development of heteroatom-doped Mo2C to fabricate a water electrolyzer is still a challenge because of the limitation of a well-defined electronic structure of hybridization of Mo with heteroatom(s). Here, nitrogen (N) and phosphor (P) codoped Mo2C embedded carbon nanotubes (NCNTP,N-Mo2C) with the priority occupation of C-sites by N, which well confines the P-implantation at the pyrrodic N-sites and brings out N-O bonding on the surface, which favorably modifies the electronic configuration of adjacent Mo, resulting in highly efficient pH-tolerant HER activity. This study not only presents a potential HER electrocatalyst candidate but also provides a strategy for the construction of a well-defined electronic structure of heteroatom(s)-neighboring carbon-based materials
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|a Journal Article
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| 700 |
1 |
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|a Cai, Mengdie
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Jiang, Yong
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wang, Qi
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wang, Azhu
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Chen, Jingshuai
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wei, Yuxue
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Cheng, Qin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Sun, Song
|e verfasserin
|4 aut
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| 773 |
0 |
8 |
|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1992
|g 38(2022), 12 vom: 29. März, Seite 3795-3803
|w (DE-627)NLM098181009
|x 1520-5827
|7 nnns
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| 773 |
1 |
8 |
|g volume:38
|g year:2022
|g number:12
|g day:29
|g month:03
|g pages:3795-3803
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| 856 |
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|u http://dx.doi.org/10.1021/acs.langmuir.1c03428
|3 Volltext
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