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231225s2022 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202200860
|2 doi
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|a pubmed24n1126.xml
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|a (DE-627)NLM337938784
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|a (NLM)35262983
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Zhang, Min
|e verfasserin
|4 aut
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|a Construction of Mixed Ionic-Electronic Conducting Scaffolds in Zn Powder
|b A Scalable Route to Dendrite-Free and Flexible Zn Anodes
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|c 2022
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|a Text
|b txt
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 16.05.2022
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2022 Wiley-VCH GmbH.
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|a Zn powder (Zn-P)-based anodes are considered ideal candidates for Zn-based batteries because they enable a positive synergistic integration of safety and energy density. However, Zn-P-based anodes still experience easy corrosion, uncontrolled dendrite growth, and poor mechanical strength, which restrict their further application. Herein, a mixed ionic-electronic conducting scaffold is introduced into Zn-P to successfully fabricate anti-corrosive, flexible, and dendrite-free Zn anodes using a scalable tape-casting strategy. The as-established scaffold is characterized by robust flexibility, facile scale-up synthesis methodology, and exceptional anti-corrosive characteristics, and it can effectively homogenize the Zn2+ flux during Zn plating/stripping, thus allowing stable Zn cycling. Benefiting from these comprehensive attributes, the as-prepared Zn-P-based anode provides superior electrochemical performance, including long-life cycling stability and high rate capability in practical coin and flexible pouch cells; thus, it holds great potential for developing advanced Zn-ion batteries. The findings of this study provide insights for a promising scalable pathway to fabricate highly efficient and reliable Zn-based anodes and will aid in the realization of advanced flexible energy-storage devices
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|a Journal Article
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|a Zn powder
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|a dendrite-free Zn anodes
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|a flexible Zn anode
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|a mixed ionic-electronic conductor
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|a Yu, Peifeng
|e verfasserin
|4 aut
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|a Xiong, Kairong
|e verfasserin
|4 aut
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|a Wang, Yongyin
|e verfasserin
|4 aut
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|a Liu, Yingliang
|e verfasserin
|4 aut
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|a Liang, Yeru
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 34(2022), 19 vom: 11. Mai, Seite e2200860
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:34
|g year:2022
|g number:19
|g day:11
|g month:05
|g pages:e2200860
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|u http://dx.doi.org/10.1002/adma.202200860
|3 Volltext
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