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231225s2022 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202104952
|2 doi
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|a pubmed24n1123.xml
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|a eng
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| 100 |
1 |
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|a Zhang, Weiyi
|e verfasserin
|4 aut
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| 245 |
1 |
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|a Macroscale Conjugated Microporous Polymers
|b Controlling Versatile Functionalities Over Several Dimensions
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|c 2022
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| 336 |
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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| 338 |
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|a ƒa Online-Ressource
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|a Date Revised 06.05.2022
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2022 The Authors. Advanced Materials published by Wiley-VCH GmbH.
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|a Since discovered in 2007, conjugated microporous polymers (CMPs) have been developed for numerous applications including gas adsorption, sensing, organic and photoredox catalysis, energy storage, etc. While featuring abundant micropores, the structural rigidity derived from CMPs' stable π-conjugated skeleton leads to insolubility and thus poor processability, which severely limits their applicability, e.g., in CMP-based devices. Hence, the development of CMPs whose structure can not only be controlled on the micro- but also on the macroscale have attracted tremendous interest. In conventional synthesis procedures, CMPs are obtained as powders, but in recent years various bottom-up synthesis strategies have been developed, which yield CMPs as thin films on substrates or as hybrid materials, allowing to span length scales from individual conjugated monomers to micro-/macrostructures. This review surveys recent advances on the construction of CMPs into macroscale structures, including membranes, films, aerogels, sponges, and other architectures. The focus is to describe the underlying fabrication techniques and the implications which follow from the macroscale morphologies, involving new chemistry and physics in such materials for applications like molecular separation/filtration/adsorption, energy storage and conversion, photothermal transformation, sensing, or catalysis
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|a Journal Article
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|a Review
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|a adsorption and separation
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| 650 |
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4 |
|a energy storage and conversion
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| 650 |
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|a heterogeneous catalysis
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| 650 |
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|a macroscale conjugated microporous polymers
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| 650 |
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4 |
|a smart materials
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1 |
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|a Zuo, Hongyu
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Cheng, Zhonghua
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Shi, Yu
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Guo, Zhengjun
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Meng, Nan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Thomas, Arne
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Liao, Yaozu
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 34(2022), 18 vom: 21. Mai, Seite e2104952
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|g volume:34
|g year:2022
|g number:18
|g day:21
|g month:05
|g pages:e2104952
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|u http://dx.doi.org/10.1002/adma.202104952
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