Highly Conducting and Stretchable Double-Network Hydrogel for Soft Bioelectronics

© 2022 Wiley-VCH GmbH.

Détails bibliographiques
Publié dans:Advanced materials (Deerfield Beach, Fla.). - 1998. - 34(2022), 15 vom: 15. Apr., Seite e2200261
Auteur principal: Li, Gang (Auteur)
Autres auteurs: Huang, Kaixi, Deng, Jue, Guo, Mengxue, Cai, Minkun, Zhang, Yuan, Guo, Chuan Fei
Format: Article en ligne
Langue:English
Publié: 2022
Accès à la collection:Advanced materials (Deerfield Beach, Fla.)
Sujets:Journal Article PEDOT:PSS conducting polymers double-network hydrogels electrode-tissue integration in situ aggregation Adhesives Hydrogels Polymers
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520 |a Conducting polymer hydrogels are promising materials in soft bioelectronics because of their tissue-like mechanical properties and the capability of electrical interaction with tissues. However, it is challenging to balance electrical conductivity and mechanical stretchability: pure conducting polymer hydrogels are highly conductive, but they are brittle; while incorporating the conducting network with a soft network to form a double network can improve the stretchability, its electrical conductivity significantly decreases. Here, the problem is addressed by concentrating a poorly crosslinked precursor hydrogel with a high content ratio of the conducting polymer to achieve a densified double-network hydrogel (5.5 wt% conducting polymer), exhibiting both high electrical conductivity (≈10 S cm-1 ) and a large fracture strain (≈150%), in addition to high biocompatibility, tissue-like softness, low swelling ratio, and desired electrochemical properties for bioelectronics. A surface grafting method is further used to form an adhesive layer on the conducting hydrogel, enabling robust and rapid bonding on the tissues. Furthermore, the proposed hydrogel is applied to show high-quality physiological signal recording and reliable, low-voltage electrical stimulation based on an in vivo rat model. This method provides an ideal strategy for rapid and reliable tissue-device integration with high-quality electrical communications 
650 4 |a Journal Article 
650 4 |a PEDOT:PSS 
650 4 |a conducting polymers 
650 4 |a double-network hydrogels 
650 4 |a electrode-tissue integration 
650 4 |a in situ aggregation 
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650 7 |a Hydrogels  |2 NLM 
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700 1 |a Huang, Kaixi  |e verfasserin  |4 aut 
700 1 |a Deng, Jue  |e verfasserin  |4 aut 
700 1 |a Guo, Mengxue  |e verfasserin  |4 aut 
700 1 |a Cai, Minkun  |e verfasserin  |4 aut 
700 1 |a Zhang, Yuan  |e verfasserin  |4 aut 
700 1 |a Guo, Chuan Fei  |e verfasserin  |4 aut 
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