Degradation of refractory organic matter in the effluent from a semi-aerobic aged refuse biofilter-treated landfill leachate by a nano-Fe3O4 enhanced ozonation process

In this study, the transformation and degradation mechanisms of refractory organic matter in biologically treated leachate from a semi-aerobic aged refuse biofilter (SAARB) in a nano-Fe3O4 enhanced ozonation process (nFe3O4-O3) were investigated in batch experiments. A continuous experiment then con...

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Veröffentlicht in:Waste management & research : the journal of the International Solid Wastes and Public Cleansing Association, ISWA. - 1991. - 40(2022), 8 vom: 30. Aug., Seite 1242-1255
1. Verfasser: Huang, Yuyu (VerfasserIn)
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2022
Zugriff auf das übergeordnete Werk:Waste management & research : the journal of the International Solid Wastes and Public Cleansing Association, ISWA
Schlagworte:Journal Article Semi-aerobic aged refuse biofilter advanced oxidation process continuous ozonation humic substances removal refractory organic matter Ferric Compounds Water Pollutants, Chemical ferric oxide 1K09F3G675 mehr... Ozone 66H7ZZK23N
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245 1 0 |a Degradation of refractory organic matter in the effluent from a semi-aerobic aged refuse biofilter-treated landfill leachate by a nano-Fe3O4 enhanced ozonation process 
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500 |a Date Completed 17.06.2022 
500 |a Date Revised 28.06.2022 
500 |a published: Print-Electronic 
500 |a Citation Status MEDLINE 
520 |a In this study, the transformation and degradation mechanisms of refractory organic matter in biologically treated leachate from a semi-aerobic aged refuse biofilter (SAARB) in a nano-Fe3O4 enhanced ozonation process (nFe3O4-O3) were investigated in batch experiments. A continuous experiment then confirmed the effectiveness of the process for SAARB effluent treatment. In a batch experiment, the effects of influencing factors, including nFe3O4 dosage, O3 dosage and initial pH on the treatment performance of nFe3O4-O3 process, were comprehensively investigated. The results showed that when the nFe3O4 dosage = 6 g L-1, O3 dosage = 0.15 L minute-1 and initial pH = 7, the total organic carbon, absorbance at 254 nm and colour number removal efficiencies were 40.58%, 62.55% and 89.80%, respectively. In addition, most of the humic- and fulvic-like substances in the SAARB effluent were removed, and the condensation degree, aromaticity and humification degree of the organics were substantially reduced. The morphology and elemental valence state analysis showed that the nFe3O4 in the process was relatively stable and could form an nFe3O4-organic complex. Therefore, the probability of organics reacting with hydroxyl radical increased and the oxidation efficiency was enhanced. In the continuous experiment, both the O3 dosage and hydraulic retention time (HRT) were the key influencing factors. The treatment efficiency of the nFe3O4-O3 process was enhanced at a higher O3 dosage and longer HRT. The electrical energy consumption of the continuous nFe3O3-O3 process was calculated to be 17.72 kW h m-3 in SAARB effluent treatment. This study proved the feasibility of biologically treated landfill leachate treatment by the nFe3O3-O3 process 
650 4 |a Journal Article 
650 4 |a Semi-aerobic aged refuse biofilter 
650 4 |a advanced oxidation process 
650 4 |a continuous ozonation 
650 4 |a humic substances removal 
650 4 |a refractory organic matter 
650 7 |a Ferric Compounds  |2 NLM 
650 7 |a Water Pollutants, Chemical  |2 NLM 
650 7 |a ferric oxide  |2 NLM 
650 7 |a 1K09F3G675  |2 NLM 
650 7 |a Ozone  |2 NLM 
650 7 |a 66H7ZZK23N  |2 NLM 
773 0 8 |i Enthalten in  |t Waste management & research : the journal of the International Solid Wastes and Public Cleansing Association, ISWA  |d 1991  |g 40(2022), 8 vom: 30. Aug., Seite 1242-1255  |w (DE-627)NLM098164791  |x 1096-3669  |7 nnns 
773 1 8 |g volume:40  |g year:2022  |g number:8  |g day:30  |g month:08  |g pages:1242-1255 
856 4 0 |u http://dx.doi.org/10.1177/0734242X211066229  |3 Volltext 
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