Multiferroic-Enabled Magnetic-Excitons in 2D Quantum-Entangled Van der Waals Antiferromagnet NiI2

© 2022 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 34(2022), 10 vom: 01. März, Seite e2109144
1. Verfasser: Son, Suhan (VerfasserIn)
Weitere Verfasser: Lee, Youjin, Kim, Jae Ha, Kim, Beom Hyun, Kim, Chaebin, Na, Woongki, Ju, Hwiin, Park, Sudong, Nag, Abhishek, Zhou, Ke-Jin, Son, Young-Woo, Kim, Hyeongdo, Noh, Woo-Suk, Park, Jae-Hoon, Lee, Jong Seok, Cheong, Hyeonsik, Kim, Jae Hoon, Park, Je-Geun
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2022
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article Zhang-Rice singlet states Zhang-Rice triplet states multiferroic van der Waals NiI2 optical absorption quantum entanglement second-harmonic generation
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520 |a Matter-light interaction is at the center of diverse research fields from quantum optics to condensed matter physics, opening new fields like laser physics. A magnetic exciton is one such rare example found in magnetic insulators. However, it is relatively rare to observe that external variables control matter-light interaction. Here, it is reported that the broken inversion symmetry of multiferroicity can act as an external knob enabling magnetic excitons in the van der Waals antiferromagnet NiI2 . It is further discovered that this magnetic exciton arises from a transition between Zhang-Rice-triplet and Zhang-Rice-singlet fundamentally quantum-entangled states. This quantum entanglement produces an ultrasharp optical exciton peak at 1.384 eV with a 5 meV linewidth. The work demonstrates that NiI2 is 2D magnetically ordered with an intrinsically quantum-entangled ground state 
650 4 |a Journal Article 
650 4 |a Zhang-Rice singlet states 
650 4 |a Zhang-Rice triplet states 
650 4 |a multiferroic van der Waals NiI2 
650 4 |a optical absorption 
650 4 |a quantum entanglement 
650 4 |a second-harmonic generation 
700 1 |a Lee, Youjin  |e verfasserin  |4 aut 
700 1 |a Kim, Jae Ha  |e verfasserin  |4 aut 
700 1 |a Kim, Beom Hyun  |e verfasserin  |4 aut 
700 1 |a Kim, Chaebin  |e verfasserin  |4 aut 
700 1 |a Na, Woongki  |e verfasserin  |4 aut 
700 1 |a Ju, Hwiin  |e verfasserin  |4 aut 
700 1 |a Park, Sudong  |e verfasserin  |4 aut 
700 1 |a Nag, Abhishek  |e verfasserin  |4 aut 
700 1 |a Zhou, Ke-Jin  |e verfasserin  |4 aut 
700 1 |a Son, Young-Woo  |e verfasserin  |4 aut 
700 1 |a Kim, Hyeongdo  |e verfasserin  |4 aut 
700 1 |a Noh, Woo-Suk  |e verfasserin  |4 aut 
700 1 |a Park, Jae-Hoon  |e verfasserin  |4 aut 
700 1 |a Lee, Jong Seok  |e verfasserin  |4 aut 
700 1 |a Cheong, Hyeonsik  |e verfasserin  |4 aut 
700 1 |a Kim, Jae Hoon  |e verfasserin  |4 aut 
700 1 |a Park, Je-Geun  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Advanced materials (Deerfield Beach, Fla.)  |d 1998  |g 34(2022), 10 vom: 01. März, Seite e2109144  |w (DE-627)NLM098206397  |x 1521-4095  |7 nnns 
773 1 8 |g volume:34  |g year:2022  |g number:10  |g day:01  |g month:03  |g pages:e2109144 
856 4 0 |u http://dx.doi.org/10.1002/adma.202109144  |3 Volltext 
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