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231225s2022 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202104405
|2 doi
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|a pubmed24n1108.xml
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|a (DE-627)NLM332645134
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|a (NLM)34726305
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|a DE-627
|b ger
|c DE-627
|e rakwb
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| 041 |
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|a eng
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| 100 |
1 |
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|a Nai, Jianwei
|e verfasserin
|4 aut
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| 245 |
1 |
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|a Construction of Ni(CN)2 /NiSe2 Heterostructures by Stepwise Topochemical Pathways for Efficient Electrocatalytic Oxygen Evolution
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|c 2022
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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| 338 |
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 27.01.2022
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2021 Wiley-VCH GmbH.
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|a Exploiting effective electrocatalysts based on elaborate heterostructures for the oxygen evolution reaction (OER) has been considered as a promising strategy for boosting water splitting efficiency to produce the clean energy-hydrogen. However, constructing catalytically active heterostructures with novel composition and architecture remains poorly developed due to the synthetic challenge. In this work, it is demonstrated that unique Ni(CN)2 /NiSe2 heterostructures, composed of single-crystalline Ni(CN)2 nanoplates surrounded by crystallographically aligned NiSe2 nanosatellites, can be created from nickel-based Hofmann-type coordination polymers through stepwise topochemical pathways. When employed as the OER electrocatalyst, the Ni(CN)2 /NiSe2 heterostructures show enhanced performance, which could be attributed to optimized geometric and electronic structures of the catalytic sites endowed by the synergy between the two components. This work demonstrates a rational synthetic route for creating a novel Ni-based OER electrocatalyst that possesses nanoscale heterostructure, whose composition, spatial organization, and interface configuration can be finely manipulated
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4 |
|a Journal Article
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| 650 |
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4 |
|a electrocatalysts
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| 650 |
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4 |
|a heterostructures
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| 650 |
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4 |
|a nanostructures
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| 650 |
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4 |
|a oxygen evolution reaction
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| 650 |
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4 |
|a topochemical reactions
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| 700 |
1 |
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|a Xu, Xiangzhen
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Xie, Qifan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Lu, Gongxun
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wang, Yao
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Luan, Deyan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Tao, Xinyong
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Lou, Xiong Wen David
|e verfasserin
|4 aut
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| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 34(2022), 4 vom: 05. Jan., Seite e2104405
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
1 |
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|g volume:34
|g year:2022
|g number:4
|g day:05
|g month:01
|g pages:e2104405
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| 856 |
4 |
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|u http://dx.doi.org/10.1002/adma.202104405
|3 Volltext
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