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231225s2021 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202106627
|2 doi
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|a pubmed24n1105.xml
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|a (DE-627)NLM331735563
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|a (NLM)34632639
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|a DE-627
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|c DE-627
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|a eng
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|a Salcedo-Abraira, Pablo
|e verfasserin
|4 aut
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|a A Novel Porous Ti-Squarate as Efficient Photocatalyst in the Overall Water Splitting Reaction under Simulated Sunlight Irradiation
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|c 2021
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 28.12.2021
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2021 Wiley-VCH GmbH.
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|a A new porous titanium(IV) squarate metal-organic framework (MOF), denoted as IEF-11, having a never reported titanium secondary building unit, is successfully synthesized and fully characterized. IEF-11 not only exhibits a permanent porosity but also an outstanding chemical stability. Further, as a consequence of combining the photoactive Ti(IV) and the electroactive squarate, IEF-11 presents relevant optoelectronic properties, applied here to the photocatalytic overall water splitting reaction. Remarkably, IEF-11 as a photocatalyst is able to produce record H2 amounts for MOF-based materials under simulated sunlight (up to 672 µmol gcatalyst in 22 h) without any activity loss during at least 10 d
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|a Journal Article
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|a metal-organic frameworks
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|a porosity
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|a titanium
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|a water splitting photocatalysis
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|a Babaryk, Artem A
|e verfasserin
|4 aut
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|a Montero-Lanzuela, Eva
|e verfasserin
|4 aut
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|a Contreras-Almengor, Oscar R
|e verfasserin
|4 aut
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|a Cabrero-Antonino, María
|e verfasserin
|4 aut
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|a Grape, Erik Svensson
|e verfasserin
|4 aut
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|a Willhammar, Tom
|e verfasserin
|4 aut
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|a Navalón, Sergio
|e verfasserin
|4 aut
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| 700 |
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|a Elkäim, Erik
|e verfasserin
|4 aut
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| 700 |
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|a García, Hermenegildo
|e verfasserin
|4 aut
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| 700 |
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|a Horcajada, Patricia
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 33(2021), 52 vom: 11. Dez., Seite e2106627
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:33
|g year:2021
|g number:52
|g day:11
|g month:12
|g pages:e2106627
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|u http://dx.doi.org/10.1002/adma.202106627
|3 Volltext
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|d 33
|j 2021
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|h e2106627
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