Efficient Organic Upconversion Devices for Low Energy Consumption and High-Quality Noninvasive Imaging

© 2021 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 33(2021), 42 vom: 17. Okt., Seite e2102812
1. Verfasser: Du, Xiaoyang (VerfasserIn)
Weitere Verfasser: Han, Jiayue, He, Zeyu, Han, Chao, Wang, Xiaomu, Wang, Jun, Jiang, Yadong, Tao, Silu
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2021
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article imaging linear dynamic range low energy consumption near-infrared photodetection noninvasive imaging organic upconversion devices Coordination Complexes Organic Chemicals
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520 |a Infrared upconversion devices (UCDs) enable low-cost visualization of infrared optical signals without utilizing a readout circuit, which is of great significance for biological recognition and noninvasive dynamic monitoring. However, UCDs suffer from inferior photon to photon (p-p) efficiency and high turn-on voltage (Von ) for upconversion operation, hindering a further expansion in highly resolved infrared imaging. Herein, an efficient organic UCD integrating an interfacial exciplex emitter and a well-designed near-infrared (NIR) detector reveals a high efficiency up to 12.92% and a low Von down to 1.56 V. The low Von gives the capacity for detecting weak NIR light down to 3.2 µW cm-2 , significantly expanding the detection power scale of UCDs. Thus, the imaging linear dynamic range (I-LDR) is highly bias-tunable, ranging from 13.23 to 84.4 dB. The high I-LDR enables highly resolved and strong-penetration bioimaging especially for thick biological sections, indicating great potential in noninvasive defect and pathological detection 
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650 4 |a imaging linear dynamic range 
650 4 |a low energy consumption 
650 4 |a near-infrared photodetection 
650 4 |a noninvasive imaging 
650 4 |a organic upconversion devices 
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700 1 |a Han, Jiayue  |e verfasserin  |4 aut 
700 1 |a He, Zeyu  |e verfasserin  |4 aut 
700 1 |a Han, Chao  |e verfasserin  |4 aut 
700 1 |a Wang, Xiaomu  |e verfasserin  |4 aut 
700 1 |a Wang, Jun  |e verfasserin  |4 aut 
700 1 |a Jiang, Yadong  |e verfasserin  |4 aut 
700 1 |a Tao, Silu  |e verfasserin  |4 aut 
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