A High-Efficiency Wavelength-Tunable Monolayer LED with Hybrid Continuous-Pulsed Injection

© 2021 Wiley-VCH GmbH.

Détails bibliographiques
Publié dans:Advanced materials (Deerfield Beach, Fla.). - 1998. - 33(2021), 29 vom: 15. Juli, Seite e2101375
Auteur principal: Zhu, Yi (Auteur)
Autres auteurs: Wang, Bowen, Li, Ziyuan, Zhang, Jian, Tang, Yilin, Torres, Juan F, Lipiński, Wojciech, Fu, Lan, Lu, Yuerui
Format: Article en ligne
Langue:English
Publié: 2021
Accès à la collection:Advanced materials (Deerfield Beach, Fla.)
Sujets:Journal Article 2D materials WS2 hybrid injection light-emitting diodes wavelength-tunability
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520 |a High-efficiency and wavelength-tunable light-emitting diode (LED) devices will play an important role in future advanced optoelectronic systems. Traditional semiconductor LED devices typically have a fixed emission wavelength that is determined by the energy of the emission states. Here, a novel high-efficiency and wavelength-tunable monolayer WS2 LED device, which operates in the hybrid mode of continuous-pulsed injection, is developed. This hybrid injection enables highly enhanced emission efficiency (>20 times) and effective size of emission area (>5 times) at room temperature. The emission wavelength of the WS2 monolayer LED device can be tuned over more than 40 nm by driving AC voltages, from exciton emission to trion emission, and further to defect emission. The quantum efficiency of defect electroluminescence (EL) emission is measured to be more than 24.5 times larger than that from free exciton and trion EL emission. The separate carrier injection in the LED also demonstrates advantages in allowing defect species to be visualized and distinguished in real space. Those defects are assigned to be negatively charged defects. The results open a new route to develop high-performance and wavelength-tunable LED devices for future advanced optoelectronic applications 
650 4 |a Journal Article 
650 4 |a 2D materials 
650 4 |a WS2 
650 4 |a hybrid injection 
650 4 |a light-emitting diodes 
650 4 |a wavelength-tunability 
700 1 |a Wang, Bowen  |e verfasserin  |4 aut 
700 1 |a Li, Ziyuan  |e verfasserin  |4 aut 
700 1 |a Zhang, Jian  |e verfasserin  |4 aut 
700 1 |a Tang, Yilin  |e verfasserin  |4 aut 
700 1 |a Torres, Juan F  |e verfasserin  |4 aut 
700 1 |a Lipiński, Wojciech  |e verfasserin  |4 aut 
700 1 |a Fu, Lan  |e verfasserin  |4 aut 
700 1 |a Lu, Yuerui  |e verfasserin  |4 aut 
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773 1 8 |g volume:33  |g year:2021  |g number:29  |g day:15  |g month:07  |g pages:e2101375 
856 4 0 |u http://dx.doi.org/10.1002/adma.202101375  |3 Volltext 
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