Magnetic recyclable heterogeneous catalyst Fe3O4/g-C3N4 for tetracycline hydrochloride degradation via photo-Fenton process under visible light

Antibiotic pollution of water resources is a global problem, and the development of new treatments for destroying antibiotics in water is a priority research. We successfully manufactured recyclable magnetic Fe3O4/g-C3N4 through the electrostatic self-assembly method. Selecting tetracycline (TC) as...

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Veröffentlicht in:Environmental technology. - 1993. - 43(2022), 21 vom: 29. Sept., Seite 3341-3354
1. Verfasser: Cui, Kang-Ping (VerfasserIn)
Weitere Verfasser: Yang, Ting-Ting, Chen, Yi-Han, Weerasooriya, Rohan, Li, Guang-Hong, Zhou, Kai, Chen, Xing
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2022
Zugriff auf das übergeordnete Werk:Environmental technology
Schlagworte:Journal Article Fe3O4/g-C3N4 magnetic recovery photo-Fenton system tetracycline visible-light photocatalysis Anti-Bacterial Agents Water 059QF0KO0R Hydrogen Peroxide mehr... BBX060AN9V Tetracycline F8VB5M810T
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245 1 0 |a Magnetic recyclable heterogeneous catalyst Fe3O4/g-C3N4 for tetracycline hydrochloride degradation via photo-Fenton process under visible light 
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520 |a Antibiotic pollution of water resources is a global problem, and the development of new treatments for destroying antibiotics in water is a priority research. We successfully manufactured recyclable magnetic Fe3O4/g-C3N4 through the electrostatic self-assembly method. Selecting tetracycline (TC) as the target pollutant, using Fe3O4/g-C3N4 and H2O2 developed a heterogeneous optical Fenton system to remove TC under visible light. Fe3O4/g-C3N4 was systematically characterized by SEM, TEM, XRD, FTIR, XPS, DRS, and electrochemical methods. The removal efficiency of 7% Fe3O4/g-C3N4 at pH = 3, H2O2 = 5 mM, and catalyst dosage of 1.0 g/L can reach 99.8%. After magnetic separation, the Fe3O4/g-C3N4 photocatalyst can be recycled five times with minimal efficiency loss. The excellent degradation performance of the prepared catalyst may be attributed to the proper coupling interface between Fe3O4 and g-C3N4 which promotes the separation and transfer of photogenerated electrons. Photogenerated electrons can also accelerate the conversion of Fe3+ to Fe2+, thereby producing more ˙OH. The new Fe3O4/g-C3N4 can be used as a raw material for advanced oxidation of water contaminated by refractory antibiotics 
650 4 |a Journal Article 
650 4 |a Fe3O4/g-C3N4 
650 4 |a magnetic recovery 
650 4 |a photo-Fenton system 
650 4 |a tetracycline 
650 4 |a visible-light photocatalysis 
650 7 |a Anti-Bacterial Agents  |2 NLM 
650 7 |a Water  |2 NLM 
650 7 |a 059QF0KO0R  |2 NLM 
650 7 |a Hydrogen Peroxide  |2 NLM 
650 7 |a BBX060AN9V  |2 NLM 
650 7 |a Tetracycline  |2 NLM 
650 7 |a F8VB5M810T  |2 NLM 
700 1 |a Yang, Ting-Ting  |e verfasserin  |4 aut 
700 1 |a Chen, Yi-Han  |e verfasserin  |4 aut 
700 1 |a Weerasooriya, Rohan  |e verfasserin  |4 aut 
700 1 |a Li, Guang-Hong  |e verfasserin  |4 aut 
700 1 |a Zhou, Kai  |e verfasserin  |4 aut 
700 1 |a Chen, Xing  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Environmental technology  |d 1993  |g 43(2022), 21 vom: 29. Sept., Seite 3341-3354  |w (DE-627)NLM098202545  |x 1479-487X  |7 nnas 
773 1 8 |g volume:43  |g year:2022  |g number:21  |g day:29  |g month:09  |g pages:3341-3354 
856 4 0 |u http://dx.doi.org/10.1080/09593330.2021.1921052  |3 Volltext 
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