Recent Development of Oxygen Evolution Electrocatalysts in Acidic Environment

© 2021 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 33(2021), 20 vom: 07. Mai, Seite e2006328
1. Verfasser: An, Li (VerfasserIn)
Weitere Verfasser: Wei, Chao, Lu, Min, Liu, Hanwen, Chen, Yubo, Scherer, Günther G, Fisher, Adrian C, Xi, Pinxian, Xu, Zhichuan J, Yan, Chun-Hua
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2021
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article Review acidic environment catalytic activity electrocatalysis oxygen evolution reaction stability of electrocatalysts
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520 |a The proton exchange membrane (PEM) water electrolysis is one of the most promising hydrogen production techniques. The oxygen evolution reaction (OER) occurring at the anode dominates the overall efficiency. Developing active and robust electrocatalysts for OER in acid is a longstanding challenge for PEM water electrolyzers. Most catalysts show unsatisfied stability under strong acidic and oxidative conditions. Such a stability challenge also leads to difficulties for a better understanding of mechanisms. This review aims to provide the current progress on understanding of OER mechanisms in acid, analyze the promising strategies to enhance both activity and stability, and summarize the state-of-the-art catalysts for OER in acid. First, the prevailing OER mechanisms are reviewed to establish the physicochemical structure-activity relationships for guiding the design of highly efficient OER electrocatalysts in acid with stable performance. The reported approaches to improve the activity, from macroview to microview, are then discussed. To analyze the problem of instability, the key factors affecting catalyst stability are summarized and the surface reconstruction is discussed. Various noble-metal-based OER catalysts and the current progress of non-noble-metal-based catalysts are reviewed. Finally, the challenges and perspectives for the development of active and robust OER catalysts in acid are discussed 
650 4 |a Journal Article 
650 4 |a Review 
650 4 |a acidic environment 
650 4 |a catalytic activity 
650 4 |a electrocatalysis 
650 4 |a oxygen evolution reaction 
650 4 |a stability of electrocatalysts 
700 1 |a Wei, Chao  |e verfasserin  |4 aut 
700 1 |a Lu, Min  |e verfasserin  |4 aut 
700 1 |a Liu, Hanwen  |e verfasserin  |4 aut 
700 1 |a Chen, Yubo  |e verfasserin  |4 aut 
700 1 |a Scherer, Günther G  |e verfasserin  |4 aut 
700 1 |a Fisher, Adrian C  |e verfasserin  |4 aut 
700 1 |a Xi, Pinxian  |e verfasserin  |4 aut 
700 1 |a Xu, Zhichuan J  |e verfasserin  |4 aut 
700 1 |a Yan, Chun-Hua  |e verfasserin  |4 aut 
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773 1 8 |g volume:33  |g year:2021  |g number:20  |g day:07  |g month:05  |g pages:e2006328 
856 4 0 |u http://dx.doi.org/10.1002/adma.202006328  |3 Volltext 
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