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231225s2021 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202005206
|2 doi
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|a pubmed24n1076.xml
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|a (DE-627)NLM323080464
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|a (NLM)33751709
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Kusada, Kohei
|e verfasserin
|4 aut
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| 245 |
1 |
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|a Highly Stable and Active Solid-Solution-Alloy Three-Way Catalyst by Utilizing Configurational-Entropy Effect
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|c 2021
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Revised 20.04.2021
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2021 Wiley-VCH GmbH.
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|a Since 1970, people have been making every endeavor to reduce toxic emissions from automobiles. After the development of a three-way catalyst (TWC) that concurrently converts three harmful gases, carbon monoxide (CO), hydrocarbons (HCs), and nitrogen oxides (NOx ), Rh became an essential element in automobile technology because only Rh works efficiently for catalytic NOx reduction. However, due to the sharp price spike in 2007, numerous efforts have been made to replace Rh in TWCs. Nevertheless, Rh remains irreplaceable, and now, the price of Rh is increasing significantly again. Here, it is demonstrated that PdRuM ternary solid-solution alloy nanoparticles (NPs) exhibit highly durable and active TWC performance, which will result in a significant reduction in catalyst cost compared to Rh. This work provides insights into the design of highly durable and efficient functional alloy NPs, guiding how to best take advantage of the configurational entropy in addition to the mixing enthalpy
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|a Journal Article
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|a NOx reduction
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|a catalysis
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|a configurational entropy
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4 |
|a nanoparticles
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|a solid-solution alloys
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|a three-way catalysis
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|a Wu, Dongshuang
|e verfasserin
|4 aut
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|a Nanba, Yusuke
|e verfasserin
|4 aut
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|a Koyama, Michihisa
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|4 aut
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|a Yamamoto, Tomokazu
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|4 aut
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|a Tran, Xuan Quy
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|4 aut
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|a Toriyama, Takaaki
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|4 aut
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|a Matsumura, Syo
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|4 aut
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|a Ito, Ayano
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|a Sato, Katsutoshi
|e verfasserin
|4 aut
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|a Nagaoka, Katsutoshi
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|4 aut
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|a Seo, Okkyun
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|4 aut
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|a Song, Chulho
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|4 aut
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|a Chen, Yanna
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|4 aut
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|a Palina, Natalia
|e verfasserin
|4 aut
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|a Kumara, Loku Singgappulige Rosantha
|e verfasserin
|4 aut
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| 700 |
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|a Hiroi, Satoshi
|e verfasserin
|4 aut
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|a Sakata, Osami
|e verfasserin
|4 aut
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|a Kawaguchi, Shogo
|e verfasserin
|4 aut
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| 700 |
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|a Kubota, Yoshiki
|e verfasserin
|4 aut
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| 700 |
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|a Kitagawa, Hiroshi
|e verfasserin
|4 aut
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| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 33(2021), 16 vom: 10. Apr., Seite e2005206
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:33
|g year:2021
|g number:16
|g day:10
|g month:04
|g pages:e2005206
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|u http://dx.doi.org/10.1002/adma.202005206
|3 Volltext
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