Chemistry of Atmospheric Fine Particles During the COVID-19 Pandemic in a Megacity of Eastern China

© 2020. The Authors.

Détails bibliographiques
Publié dans:Geophysical research letters. - 1984. - 48(2021), 2 vom: 28. Jan., Seite 2020GL091611
Auteur principal: Liu, Lei (Auteur)
Autres auteurs: Zhang, Jian, Du, Rongguang, Teng, Xiaomi, Hu, Rui, Yuan, Qi, Tang, Shanshan, Ren, Chuanhua, Huang, Xin, Xu, Liang, Zhang, Yinxiao, Zhang, Xiaoye, Song, Congbo, Liu, Bowen, Lu, Gongda, Shi, Zongbo, Li, Weijun
Format: Article en ligne
Langue:English
Publié: 2021
Accès à la collection:Geophysical research letters
Sujets:Journal Article COVID‐19 air pollution chemical composition fine particles megacity
Description
Résumé:© 2020. The Authors.
Air pollution in megacities represents one of the greatest environmental challenges. Our observed results show that the dramatic NOx decrease (77%) led to significant O3 increases (a factor of 2) during the COVID-19 lockdown in megacity Hangzhou, China. Model simulations further demonstrate large increases of daytime OH and HO2 radicals and nighttime NO3 radical, which can promote the gas-phase reaction and nocturnal multiphase chemistry. Therefore, enhanced NO3 - and SO4 2- formation was observed during the COVID-19 lockdown because of the enhanced oxidizing capacity. The PM2.5 decrease was only partially offset by enhanced aerosol formation with its reduction reaching 50%. In particular, NO3 - decreased largely by 68%. PM2.5 chemical analysis reveals that vehicular emissions mainly contributed to PM2.5 under normal conditions in Hangzhou. Whereas, stationary sources dominated the residual PM2.5 during the COVID-19 lockdown. This study provides evidence that large reductions in vehicular emissions can effectively mitigate air pollution in megacities
Description:Date Revised 30.03.2024
published: Print-Electronic
figshare: 10.6084/m9.figshare.12919013
Citation Status PubMed-not-MEDLINE
ISSN:0094-8276
DOI:10.1029/2020GL091611