Saturation and self-absorption effects in the angle-dependent 2p3d resonant inelastic X-ray scattering spectra of Co3

open access.

Bibliographische Detailangaben
Veröffentlicht in:Journal of synchrotron radiation. - 1994. - 27(2020), Pt 4 vom: 01. Juli, Seite 979-987
1. Verfasser: Wang, Ru Pan (VerfasserIn)
Weitere Verfasser: Elnaggar, Hebatalla, Titus, Charles J, Tomiyasu, Keisuke, Geessinck, Jaap, Koster, Gertjan, Frati, Federica, Okamoto, Jun, Huang, Di Jing, de Groot, Frank M F
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Journal of synchrotron radiation
Schlagworte:Journal Article angle-dependent RIXS/RXES saturation and self-absorption effects
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520 |a Angle-dependent 2p3d resonant inelastic X-ray scattering spectra of a LaCoO3 single crystal and a 55 nm LaCoO3 film on a SrTiO3 substrate are presented. Theoretical calculation shows that, with ∼20 meV resolved Co 2p3d resonant inelastic X-ray scattering (RIXS), the excited states of the isotropic 1A1g(Oh) ground state are split by 3d spin-orbit coupling, which can be distinguished via their angular dependence. However, strong self-absorption and saturation effects distort the spectra of the LaCoO3 single crystal and limit the observation of small angular dependence. In contrast, the RIXS on 55 nm LaCoO3 shows less self-absorption effects and preserves the angular dependence of the excited states 
650 4 |a Journal Article 
650 4 |a angle-dependent RIXS/RXES 
650 4 |a saturation and self-absorption effects 
700 1 |a Elnaggar, Hebatalla  |e verfasserin  |4 aut 
700 1 |a Titus, Charles J  |e verfasserin  |4 aut 
700 1 |a Tomiyasu, Keisuke  |e verfasserin  |4 aut 
700 1 |a Geessinck, Jaap  |e verfasserin  |4 aut 
700 1 |a Koster, Gertjan  |e verfasserin  |4 aut 
700 1 |a Frati, Federica  |e verfasserin  |4 aut 
700 1 |a Okamoto, Jun  |e verfasserin  |4 aut 
700 1 |a Huang, Di Jing  |e verfasserin  |4 aut 
700 1 |a de Groot, Frank M F  |e verfasserin  |4 aut 
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