|
|
|
|
| LEADER |
01000naa a22002652 4500 |
| 001 |
NLM320112691 |
| 003 |
DE-627 |
| 005 |
20231225172902.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
231225s2021 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.202007479
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n1067.xml
|
| 035 |
|
|
|a (DE-627)NLM320112691
|
| 035 |
|
|
|a (NLM)33448048
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Chen, Xianjie
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Efficient Photocatalytic Overall Water Splitting Induced by the Giant Internal Electric Field of a g-C3 N4 /rGO/PDIP Z-Scheme Heterojunction
|
| 264 |
|
1 |
|c 2021
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Revised 17.02.2021
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2021 Wiley-VCH GmbH.
|
| 520 |
|
|
|a A graphitic carbon nitride/rGO/perylene diimide polymer (g-C3 N4 /rGO/PDIP) Z-scheme heterojunction is successfully constructed to realize high-flux charge transfer and efficient photocatalytic overall water splitting. A giant internal electric field in the Z-scheme junction is built, enabling the charge separation efficiency to be enhanced dramatically by 8.5 times. Thus, g-C3 N4 /rGO/PDIP presents an efficient and stable photocatalytic overall water splitting activity with H2 and O2 evolution rate of 15.80 and 7.80 µmol h-1 , respectively, ≈12.1 times higher than g-C3 N4 nanosheets. Meanwhile, a notable quantum efficiency of 4.94% at 420 nm and solar-to-hydrogen energy-conversion efficiency of 0.30% are achieved, prominently surpassing many reported g-C3 N4 -based photocatalysts. Briefly, this work throws light on enhancing the internal electric field by interface control to dramatically improve the photocatalytic performance
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a Z-scheme heterostructures
|
| 650 |
|
4 |
|a graphitic carbon nitride
|
| 650 |
|
4 |
|a overall water splitting
|
| 650 |
|
4 |
|a perylene diimide polymer
|
| 650 |
|
4 |
|a photocatalysis
|
| 700 |
1 |
|
|a Wang, Jun
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Chai, Yongqiang
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zhang, Zijian
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zhu, Yongfa
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 33(2021), 7 vom: 12. Feb., Seite e2007479
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:33
|g year:2021
|g number:7
|g day:12
|g month:02
|g pages:e2007479
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.202007479
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 33
|j 2021
|e 7
|b 12
|c 02
|h e2007479
|