Thermoelectric Properties of Novel Semimetals A Case Study of YbMnSb2

Thermoelectric Properties of Novel Semimetals : A Case Study of YbMnSb2

© 2020 The Authors. Advanced Materials published by Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 33(2021), 7 vom: 24. Feb., Seite e2003168
1. Verfasser: Pan, Yu (VerfasserIn)
Weitere Verfasser: Fan, Feng-Ren, Hong, Xiaochen, He, Bin, Le, Congcong, Schnelle, Walter, He, Yangkun, Imasato, Kazuki, Borrmann, Horst, Hess, Christian, Büchner, Bernd, Sun, Yan, Fu, Chenguang, Snyder, G Jeffrey, Felser, Claudia
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2021
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article 2D Fermi surfaces Dirac bands Zintl compounds anisotropy
Beschreibung
Zusammenfassung:© 2020 The Authors. Advanced Materials published by Wiley-VCH GmbH.
The emerging class of topological materials provides a platform to engineer exotic electronic structures for a variety of applications. As complex band structures and Fermi surfaces can directly benefit thermoelectric performance it is important to identify the role of featured topological bands in thermoelectrics particularly when there are coexisting classic regular bands. In this work, the contribution of Dirac bands to thermoelectric performance and their ability to concurrently achieve large thermopower and low resistivity in novel semimetals is investigated. By examining the YbMnSb2 nodal line semimetal as an example, the Dirac bands appear to provide a low resistivity along the direction in which they are highly dispersive. Moreover, because of the regular-band-provided density of states, a large Seebeck coefficient over 160 µV K-1 at 300 K is achieved in both directions, which is very high for a semimetal with high carrier concentration. The combined highly dispersive Dirac and regular bands lead to ten times increase in power factor, reaching a value of 2.1 mW m-1 K-2 at 300 K. The present work highlights the potential of such novel semimetals for unusual electronic transport properties and guides strategies towards high thermoelectric performance
Beschreibung:Date Revised 17.02.2021
published: Print-Electronic
Citation Status PubMed-not-MEDLINE
ISSN:1521-4095
DOI:10.1002/adma.202003168