Photonic Fractal Metamaterials : A Metal-Semiconductor Platform with Enhanced Volatile-Compound Sensing Performance

© 2020 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 32(2020), 50 vom: 30. Dez., Seite e2002471
1. Verfasser: Fusco, Zelio (VerfasserIn)
Weitere Verfasser: Rahmani, Mohsen, Tran-Phu, Thanh, Ricci, Chiara, Kiy, Alexander, Kluth, Patrick, Della Gaspera, Enrico, Motta, Nunzio, Neshev, Dragomir, Tricoli, Antonio
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article 3D metamaterials fractals metal-semiconductor platforms photonics plasmonics sensors
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520 |a Advance of photonics media is restrained by the lack of structuring techniques for the 3D fabrication of active materials with long-range periodicity. A methodology is reported for the engineering of tunable resonant photonic media with thickness exceeding the plasmonic near-field enhancement region by more than two orders of magnitude. The media architecture consists of a stochastically ordered distribution of plasmonic nanocrystals in a fractal scaffold of high-index semiconductors. This plasmonic-semiconductor fractal media supports the propagation of surface plasmons with drastically enhanced intensity over multiple length scales, overcoming the 2D limitations of established metasurface technologies. The fractal media are used for the fabrication of plasmonic optical gas sensors, achieving a limit of detection of 0.01 vol% at room temperature and sensitivity up to 1.9 nm vol%-1 , demonstrating almost a fivefold increase with respect to an optimized planar geometry. Beneficially to their implementation, the self-assembly mechanism of this fractal architecture allows fabrication of micrometer-thick media over surfaces of several square centimeters in a few seconds. The designable optical features and intrinsic scalability of these photonic fractal metamaterials provide ample opportunities for applications, bridging across transformation optics, sensing, and light harvesting 
650 4 |a Journal Article 
650 4 |a 3D metamaterials 
650 4 |a fractals 
650 4 |a metal-semiconductor platforms 
650 4 |a photonics 
650 4 |a plasmonics 
650 4 |a sensors 
700 1 |a Rahmani, Mohsen  |e verfasserin  |4 aut 
700 1 |a Tran-Phu, Thanh  |e verfasserin  |4 aut 
700 1 |a Ricci, Chiara  |e verfasserin  |4 aut 
700 1 |a Kiy, Alexander  |e verfasserin  |4 aut 
700 1 |a Kluth, Patrick  |e verfasserin  |4 aut 
700 1 |a Della Gaspera, Enrico  |e verfasserin  |4 aut 
700 1 |a Motta, Nunzio  |e verfasserin  |4 aut 
700 1 |a Neshev, Dragomir  |e verfasserin  |4 aut 
700 1 |a Tricoli, Antonio  |e verfasserin  |4 aut 
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773 1 8 |g volume:32  |g year:2020  |g number:50  |g day:30  |g month:12  |g pages:e2002471 
856 4 0 |u http://dx.doi.org/10.1002/adma.202002471  |3 Volltext 
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