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231225s2020 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202004798
|2 doi
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|a pubmed24n1051.xml
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|a DE-627
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|a eng
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| 100 |
1 |
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|a Fan, Ye
|e verfasserin
|4 aut
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| 245 |
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|a A Self-Healing Amalgam Interface in Metal Batteries
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|c 2020
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 26.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2020 Wiley-VCH GmbH.
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|a Poor cyclability and safety concerns caused by the uncontrollable dendrite growth and large interfacial resistance severely restrict the practical applications of metal batteries. Herein, a facile, universal strategy to fabricate ceramic and glass phase compatible, and self-healing metal anodes is proposed. Various amalgam-metal anodes (Li, Na, Zn, Al, and Mg) show a long cycle life in symmetric cells. It has been found that liquid Li amalgam shows a complete wetting with the surface of lanthanum lithium titanate electrolyte and a glass-phase solid-state electrolyte. The interfacial compatibility between the lithium metal anode and solid-state electrolyte is dramatically improved by using an in situ regenerated amalgam interface with high electron/ion dual-conductivity, obviously decreasing the anode/electrolyte interfacial impedance. The lithium-amalgam interface between the metal anode and electrolyte undergoes a reversible isothermal phase transition between solid and liquid during the cycling process at room temperature, resulting in a self-healing surface of metal anodes
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|a Journal Article
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|a amalgam
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|a metal batteries
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|a solid-state electrolytes
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1 |
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|a Tao, Tao
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Gao, Yuxuan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Deng, Chao
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Yu, Baozhi
|e verfasserin
|4 aut
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1 |
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|a Chen, Ying Ian
|e verfasserin
|4 aut
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1 |
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|a Lu, Shengguo
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Huang, Shaoming
|e verfasserin
|4 aut
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| 773 |
0 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 32(2020), 43 vom: 05. Okt., Seite e2004798
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:32
|g year:2020
|g number:43
|g day:05
|g month:10
|g pages:e2004798
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|u http://dx.doi.org/10.1002/adma.202004798
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