Large-Area Single-Crystal Graphene via Self-Organization at the Macroscale

© 2020 The Authors. Published by Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 32(2020), 45 vom: 15. Nov., Seite e2002755
1. Verfasser: Ta, Huy Quang (VerfasserIn)
Weitere Verfasser: Bachmatiuk, Alicja, Mendes, Rafael Gregorio, Perello, David J, Zhao, Liang, Trzebicka, Barbara, Gemming, Thomas, Rotkin, Slava V, Rümmeli, Mark H
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article 2D materials bilayer graphene global alignment graphene stacking order
Beschreibung
Zusammenfassung:© 2020 The Authors. Published by Wiley-VCH GmbH.
In 1665 Christiaan Huygens first noticed how two pendulums, regardless of their initial state, would synchronize.  It is now known that the universe is full of complex self-organizing systems, from neural networks to correlated materials. Here, graphene flakes, nucleated over a polycrystalline graphene film, synchronize during growth so as to ultimately yield a common crystal orientation at the macroscale. Strain and diffusion gradients are argued as the probable causes for the long-range cross-talk between flakes and the formation of a single-grain graphene layer. The work demonstrates that graphene synthesis can be advanced to control the nucleated crystal shape, registry, and relative alignment between graphene crystals for large area, that is, a single-crystal bilayer, and (AB-stacked) few-layer graphene can been grown at the wafer scale
Beschreibung:Date Revised 10.11.2020
published: Print-Electronic
Citation Status PubMed-not-MEDLINE
ISSN:1521-4095
DOI:10.1002/adma.202002755