Multifunctional Polymer-Regulated SnO2 Nanocrystals Enhance Interface Contact for Efficient and Stable Planar Perovskite Solar Cells

© 2020 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 32(2020), 43 vom: 26. Okt., Seite e2003990
1. Verfasser: You, Shuai (VerfasserIn)
Weitere Verfasser: Zeng, Haipeng, Ku, Zhiliang, Wang, Xiaoze, Wang, Zhen, Rong, Yaoguang, Zhao, Yang, Zheng, Xin, Luo, Long, Li, Lin, Zhang, Shujing, Li, Min, Gao, Xingyu, Li, Xiong
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article crystal growth interface contact perovskite solar cells regulation of SnO2 stability
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520 |a Perovskite solar cells (PSCs) have rapidly developed and achieved power conversion efficiencies of over 20% with diverse technical routes. Particularly, planar-structured PSCs can be fabricated with low-temperature (≤150 °C) solution-based processes, which is energy efficient and compatible with flexible substrates. Here, the efficiency and stability of planar PSCs are enhanced by improving the interface contact between the SnO2 electron-transport layer (ETL) and the perovskite layer. A biological polymer (heparin potassium, HP) is introduced to regulate the arrangement of SnO2 nanocrystals, and induce vertically aligned crystal growth of perovskites on top. Correspondingly, SnO2 -HP-based devices can demonstrate an average efficiency of 23.03% on rigid substrates with enhanced open-circuit voltage (VOC ) of 1.162 V and high reproducibility. Attributed to the strengthened interface binding, the devices obtain high operational stability, retaining 97% of their initial performance (power conversion efficiency, PCE > 22%) after 1000 h operation at their maximum power point under 1 sun illumination. Besides, the HP-modified SnO2 ETL exhibits promising potential for application in flexible and large-area devices 
650 4 |a Journal Article 
650 4 |a crystal growth 
650 4 |a interface contact 
650 4 |a perovskite solar cells 
650 4 |a regulation of SnO2 
650 4 |a stability 
700 1 |a Zeng, Haipeng  |e verfasserin  |4 aut 
700 1 |a Ku, Zhiliang  |e verfasserin  |4 aut 
700 1 |a Wang, Xiaoze  |e verfasserin  |4 aut 
700 1 |a Wang, Zhen  |e verfasserin  |4 aut 
700 1 |a Rong, Yaoguang  |e verfasserin  |4 aut 
700 1 |a Zhao, Yang  |e verfasserin  |4 aut 
700 1 |a Zheng, Xin  |e verfasserin  |4 aut 
700 1 |a Luo, Long  |e verfasserin  |4 aut 
700 1 |a Li, Lin  |e verfasserin  |4 aut 
700 1 |a Zhang, Shujing  |e verfasserin  |4 aut 
700 1 |a Li, Min  |e verfasserin  |4 aut 
700 1 |a Gao, Xingyu  |e verfasserin  |4 aut 
700 1 |a Li, Xiong  |e verfasserin  |4 aut 
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773 1 8 |g volume:32  |g year:2020  |g number:43  |g day:26  |g month:10  |g pages:e2003990 
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