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231225s2020 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202003990
|2 doi
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|a pubmed24n1050.xml
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|a (DE-627)NLM315259175
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|a (NLM)32954577
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a You, Shuai
|e verfasserin
|4 aut
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|a Multifunctional Polymer-Regulated SnO2 Nanocrystals Enhance Interface Contact for Efficient and Stable Planar Perovskite Solar Cells
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|c 2020
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Revised 26.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2020 Wiley-VCH GmbH.
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|a Perovskite solar cells (PSCs) have rapidly developed and achieved power conversion efficiencies of over 20% with diverse technical routes. Particularly, planar-structured PSCs can be fabricated with low-temperature (≤150 °C) solution-based processes, which is energy efficient and compatible with flexible substrates. Here, the efficiency and stability of planar PSCs are enhanced by improving the interface contact between the SnO2 electron-transport layer (ETL) and the perovskite layer. A biological polymer (heparin potassium, HP) is introduced to regulate the arrangement of SnO2 nanocrystals, and induce vertically aligned crystal growth of perovskites on top. Correspondingly, SnO2 -HP-based devices can demonstrate an average efficiency of 23.03% on rigid substrates with enhanced open-circuit voltage (VOC ) of 1.162 V and high reproducibility. Attributed to the strengthened interface binding, the devices obtain high operational stability, retaining 97% of their initial performance (power conversion efficiency, PCE > 22%) after 1000 h operation at their maximum power point under 1 sun illumination. Besides, the HP-modified SnO2 ETL exhibits promising potential for application in flexible and large-area devices
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|a Journal Article
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|a crystal growth
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|a interface contact
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|a perovskite solar cells
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|a regulation of SnO2
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|a stability
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|a Zeng, Haipeng
|e verfasserin
|4 aut
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|a Ku, Zhiliang
|e verfasserin
|4 aut
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|a Wang, Xiaoze
|e verfasserin
|4 aut
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|a Wang, Zhen
|e verfasserin
|4 aut
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|a Rong, Yaoguang
|e verfasserin
|4 aut
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|a Zhao, Yang
|e verfasserin
|4 aut
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|a Zheng, Xin
|e verfasserin
|4 aut
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|a Luo, Long
|e verfasserin
|4 aut
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|a Li, Lin
|e verfasserin
|4 aut
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|a Zhang, Shujing
|e verfasserin
|4 aut
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|a Li, Min
|e verfasserin
|4 aut
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|a Gao, Xingyu
|e verfasserin
|4 aut
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|a Li, Xiong
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 32(2020), 43 vom: 26. Okt., Seite e2003990
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:32
|g year:2020
|g number:43
|g day:26
|g month:10
|g pages:e2003990
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|u http://dx.doi.org/10.1002/adma.202003990
|3 Volltext
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|a GBV_ILN_350
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|a AR
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|d 32
|j 2020
|e 43
|b 26
|c 10
|h e2003990
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