Microwave Hydrothermally Synthesized Metal-Organic Framework-5 Derived C-doped ZnO with Enhanced Photocatalytic Degradation of Rhodamine B

C-doped ZnO particles have been successfully prepared by the calcination using microwave hydrothermally prepared metal-organic framework-5 (MOF-5) as the precursor. MOF-5 was turned into C-doped ZnO through calcination at 500 °C, and its cubic shape was well-maintained. X-ray photoelectron spectrosc...

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Publié dans:Langmuir : the ACS journal of surfaces and colloids. - 1985. - 36(2020), 33 vom: 25. Aug., Seite 9658-9667
Auteur principal: Wang, Yingming (Auteur)
Autres auteurs: Ge, Shengsong, Cheng, Wei, Hu, Zunju, Shao, Qian, Wang, Xiaojing, Lin, Jing, Dong, Mengyao, Wang, Junxiang, Guo, Zhanhu
Format: Article en ligne
Langue:English
Publié: 2020
Accès à la collection:Langmuir : the ACS journal of surfaces and colloids
Sujets:Journal Article
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Résumé:C-doped ZnO particles have been successfully prepared by the calcination using microwave hydrothermally prepared metal-organic framework-5 (MOF-5) as the precursor. MOF-5 was turned into C-doped ZnO through calcination at 500 °C, and its cubic shape was well-maintained. X-ray photoelectron spectroscopic studies confirmed the C-doping in the ZnO. The as-prepared C-doped ZnO demonstrated a Rhodamine B (RhB) degradation efficiency of 98% in 2 h under an solar-simulated light irradiation, much higher than that of C-doped ZnO derived from MOF-5 synthesized by the ordinary hydrothermal method. The trapping experiment revealed that the crucial factors in the RhB removal were photogenerated h+ and •O2-
Description:Date Revised 25.08.2020
published: Print-Electronic
Citation Status PubMed-not-MEDLINE
ISSN:1520-5827
DOI:10.1021/acs.langmuir.0c00395