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231225s2020 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202002893
|2 doi
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|a pubmed24n1038.xml
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|a (DE-627)NLM311457568
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|a (NLM)32567132
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|a DE-627
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|c DE-627
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|a eng
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|a Meng, Linxing
|e verfasserin
|4 aut
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|a Designing a Transparent CdIn2 S4 /In2 S3 Bulk-Heterojunction Photoanode Integrated with a Perovskite Solar Cell for Unbiased Water Splitting
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|c 2020
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 16.11.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a The integration of photoelectrochemical photoanodes and solar cells to build an unbiased solar-to-hydrogen (STH) conversion system provides a promising way to solve the energy crisis. The key point is to develop highly transparent photoanodes, while its bulk separation efficiency (ηsep. ) and surface injection efficiency are as high as possible. To resolve this contradiction, first a novel CdIn2 S4 /In2 S3 bulk heterojunctions in the interior of nanosheets is designed as a photoanode with high transparency and an ultrahigh ηsep. up to 90%. Furthermore, decorating the ultrathin amorphous SnO2 layer by atomic layer deposition, the surface oxygen-evolution kinetics of the photoanode are increased significantly. As a result, the onset potential of the photoanode shifts negatively to 0.02 V vs RHE, and the photocurrent density boosts to 2.98 mA cm-2 at 1.23 V vs RHE, which is ten times higher than that of pristine CdIn2 S4 . Such a high-performance photoanode enables the integrated metal sulfide photoanode-perovskite solar cell system to deliver a STH conversion efficiency of 3.3%
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|a Journal Article
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|a atomic layer deposition
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|a bulk heterojunctions
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|a photoelectrochemical cells
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|a water splitting
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|a Wang, Min
|e verfasserin
|4 aut
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|a Sun, Haoxuan
|e verfasserin
|4 aut
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|a Tian, Wei
|e verfasserin
|4 aut
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|a Xiao, Chenhong
|e verfasserin
|4 aut
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|a Wu, Shaolong
|e verfasserin
|4 aut
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|a Cao, Fengren
|e verfasserin
|4 aut
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|a Li, Liang
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 32(2020), 30 vom: 03. Juli, Seite e2002893
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:32
|g year:2020
|g number:30
|g day:03
|g month:07
|g pages:e2002893
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|u http://dx.doi.org/10.1002/adma.202002893
|3 Volltext
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